CHARGED-PHONON ABSORPTION IN DOPED C-60

被引:111
作者
RICE, MJ
CHOI, HY
机构
[1] Materials Research Laboratory, Xerox Webster Research Center, Webster
来源
PHYSICAL REVIEW B | 1992年 / 45卷 / 17期
关键词
D O I
10.1103/PhysRevB.45.10173
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We interpret the giant infrared resonances observed in A6C60 (A = K, Rb) by Fu et al. as being due to a classic charged-phonon effect in which the T1u molecular vibration modes of C60 acquire electronic oscillator strength via coupling to virtual t1u --> t1g electronic transitions. For the compounds AxC60 (x = 3, 4, and 6), we predict, for weak electron-molecular-vibration coupling, that the softenings of the T1u modes are proportional to x, but that the integrated oscillator strengths of their absorption bands are proportional to the square of x.
引用
收藏
页码:10173 / 10176
页数:4
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