REDUCTION OF NITROGEN-OXIDES FROM POSTCOMBUSTION GASES UTILIZING MOLECULAR RADICAL SPECIES

被引:14
作者
BOYLE, J [1 ]
RUSSELL, A [1 ]
YAO, SC [1 ]
ZHOU, Q [1 ]
EKMANN, J [1 ]
FU, Y [1 ]
MATHUR, M [1 ]
机构
[1] US DOE,PITTSBURGH ENERGY TECHNOL CTR,PITTSBURGH,PA 15236
关键词
NITROGEN; COMBUSTION; KINETICS;
D O I
10.1016/0016-2361(93)90418-2
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Plasma induced radicals from ammonia, methane and hydrogen have been injected into NO laden post-combustion gases to reduce pollutant concentrations. Results of chemical kinetics modelling indicate that radicals from ammonia, which are formed by interaction with an argon plasma stream, introduced into the post-combustion gases, will provide nearly complete NO removal. Laboratory investigations have shown that molecular radical reduction is capable of providing up to 94 mol% NO reduction. Streams of ammonia or combined ammonia/methane, which provide this reduction, utilize a minimum input energy and yield no substantial ammonia discharge.
引用
收藏
页码:1419 / 1427
页数:9
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