FEMTOSECOND STUDIES OF INTERFACIAL ELECTRON-HOLE RECOMBINATION IN AQUEOUS CDS COLLOIDS

被引:26
作者
ZHANG, JZ
ONEIL, RH
ROBERTI, TW
机构
[1] Department of Chemistry and Biochemistry, University of California, Santa Cruz
关键词
D O I
10.1063/1.111986
中图分类号
O59 [应用物理学];
学科分类号
摘要
We report the measurements of the electron-hole recombination rate in aqueous CdS colloids on the femtosecond time scale. A fast 2-ps decay and a slower 45-ps decay have been observed, and the decay dynamics are found to be very sensitive to the excitation laser intensity. Geminate electron-hole recombination, responsible for the 45-ps decay, dominates the decay process at low excitation intensities, while nongeminate recombination, accounting for the 2-ps decay, becomes more important at high excitation intensities.
引用
收藏
页码:1989 / 1991
页数:3
相关论文
共 31 条
[1]   ELECTRONIC-STRUCTURE AND PHOTOEXCITED-CARRIER DYNAMICS IN NANOMETER-SIZE CDSE CLUSTERS [J].
BAWENDI, MG ;
WILSON, WL ;
ROTHBERG, L ;
CARROLL, PJ ;
JEDJU, TM ;
STEIGERWALD, ML ;
BRUS, LE .
PHYSICAL REVIEW LETTERS, 1990, 65 (13) :1623-1626
[3]   LUMINESCENCE AND PHOTOPHYSICS OF CDS SEMICONDUCTOR CLUSTERS - THE NATURE OF THE EMITTING ELECTRONIC STATE [J].
CHESTNOY, N ;
HARRIS, TD ;
HULL, R ;
BRUS, LE .
JOURNAL OF PHYSICAL CHEMISTRY, 1986, 90 (15) :3393-3399
[4]   SEMICONDUCTOR NANOCRYSTALS COVALENTLY BOUND TO METAL-SURFACES WITH SELF-ASSEMBLED MONOLAYERS [J].
COLVIN, VL ;
GOLDSTEIN, AN ;
ALIVISATOS, AP .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1992, 114 (13) :5221-5230
[5]   EVIDENCE OF STRONG AUGER RECOMBINATION IN SEMICONDUCTOR-DOPED GLASSES [J].
DEROUGEMONT, F ;
FREY, R ;
ROUSSIGNOL, P ;
RICARD, D ;
FLYTZANIS, C .
APPLIED PHYSICS LETTERS, 1987, 50 (23) :1619-1621
[6]   COLLOIDAL ZN1-XCDXS - OPTICAL SATURATION OF THE EXCITON BAND AND PRIMARY PHOTOCHEMISTRY STUDIED BY SUBPICOSECOND LASER FLASH-PHOTOLYSIS [J].
ERNSTING, NP ;
KASCHKE, M ;
WELLER, H ;
KATSIKAS, L .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 1990, 7 (08) :1630-1637
[7]   HETEROGENEOUS PHOTOCATALYSIS [J].
FOX, MA ;
DULAY, MT .
CHEMICAL REVIEWS, 1993, 93 (01) :341-357
[8]  
GHANASSI M, 1992, APPL PHYS LETT, V62, P78
[9]  
GRATZEL M, 1982, J PHYS CHEM-US, V86, P2964
[10]  
Gratzel M., 1989, HETEROGENEOUS PHOTOC