COOPERATIVE RADIATIVE DECAY OF DISORDERED MOLECULAR MONOLAYERS

被引:6
作者
WANG, NJ [1 ]
CHERNYAK, V [1 ]
MUKAMEL, S [1 ]
机构
[1] UNIV ROCHESTER, DEPT PHYS, ROCHESTER, NY 14627 USA
关键词
D O I
10.1103/PhysRevB.50.5609
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The time-resolved spontaneous emission from a disordered molecular monolayer is calculated using Green-function techniques. In addition to a fast-decaying transmitted and reflected coherent component in the forward direction, and a slowly decaying, incoherent, spatially homogeneous background, we predict a backscattering peak related to weak localization of excitons. Analytical and numerical calculations of the energy- and disorder-dependent cooperative radiative decay rate, the quantum yield of the coherent and incoherent components, and the exciton diffusion coefficient are presented.
引用
收藏
页码:5609 / 5619
页数:11
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