COLLECTIVE EXCITATIONS IN OPEN-SHELL METAL-CLUSTERS - THE TIME-DEPENDENT LOCAL-DENSITY APPROXIMATION APPLIED TO THE SELF-CONSISTENT SPHEROIDAL JELLIUM PARTICLE

被引：92

作者：

EKARDT, W

PENZAR, Z

机构：

[1] Fritz-Haber-Institut der Max-Planck-Gesellschaft, D-1000 Berlin 33

来源：

PHYSICAL REVIEW B | 1991年 / 43卷 / 02期

关键词：

D O I：

10.1103/PhysRevB.43.1322

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

The self-consistent and microscopic time-dependent local-density-approximation (TDLDA) formalism for the calculation of the dynamical electronic response properties of open-shell, axially deformed small metal clusters is presented in detail. The model is based on the self-consistent ground-state calculation of the spheroidal jellium model, giving the optimized cluster shape, driven by its open-valence-shell electronic structure. First results on the static and dynamical electronic polarizability of the strongly axially deformed Na10 cluster are reported and compared with the experimental polarizability and photoabsorption cross-section results. The variety of the future applications of the model is outlined, as well as the possible improvement of the formalism.

引用

页码：1322 / 1330

页数：9

共 29 条

[1] Abramowitz M., 1964, HDB MATH FUNCTIONS
[2] SELF-CONSISTENT CALCULATION OF THE ELECTRONIC-STRUCTURE OF SMALL JELLIUM SPHERES
BECK, DE
[J]. SOLID STATE COMMUNICATIONS, 1984, 49 (04) : 381 - 385
[3] SELF-CONSISTENT CALCULATION OF THE EIGENFREQUENCIES FOR THE ELECTRONIC EXCITATIONS IN SMALL JELLIUM SPHERES
BECK, DE
[J]. PHYSICAL REVIEW B, 1987, 35 (14): : 7325 - 7333
[4] APPLICATION OF SUM-RULES TO THE RESPONSE OF SMALL METAL PARTICLES
BERTSCH, G
EKARDT, W
[J]. PHYSICAL REVIEW B, 1985, 32 (12): : 7659 - 7663
[5] THERMAL LINE BROADENING IN SMALL METAL-CLUSTERS
BERTSCH, GF
TOMANEK, D
[J]. PHYSICAL REVIEW B, 1989, 40 (05): : 2749 - 2751
[6] TOTAL ENERGIES, ABUNDANCES, AND ELECTRONIC SHELL STRUCTURE OF LITHIUM, SODIUM, AND POTASSIUM CLUSTERS
CHOU, MY
CLELAND, A
COHEN, ML
[J]. SOLID STATE COMMUNICATIONS, 1984, 52 (07) : 645 - 648
[7] COLLECTIVE DIPOLE OSCILLATIONS IN SMALL SODIUM CLUSTERS
DEHEER, WA
SELBY, K
KRESIN, V
MASUI, J
VOLLMER, M
CHATELAIN, A
KNIGHT, WD
[J]. PHYSICAL REVIEW LETTERS, 1987, 59 (16) : 1805 - 1808
[8] COLLECTIVE MULTIPOLE EXCITATIONS IN SMALL METAL PARTICLES - CRITICAL ANGULAR-MOMENTUM LCR FOR THE EXISTENCE OF COLLECTIVE SURFACE-MODES
EKARDT, W
[J]. PHYSICAL REVIEW B, 1985, 32 (04): : 1961 - 1970
[9] SIZE-DEPENDENT PHOTOABSORPTION AND PHOTOEMISSION OF SMALL METAL PARTICLES
EKARDT, W
[J]. PHYSICAL REVIEW B, 1985, 31 (10): : 6360 - 6370
[10] STATIC POLARIZABILITY OF METAL-CLUSTERS AND THE RELATED BLUE SHIFT OF THE DIPOLAR SURFACE-PLASMON
EKARDT, W
THOAI, DBT
FRANK, F
SCHULZE, W
[J]. SOLID STATE COMMUNICATIONS, 1983, 46 (07) : 571 - 574

← 1 2 3 →