AUTOMATED MULTIDIMENSIONAL COHERENT OPTICAL SPECTROSCOPY WITH MULTIPLE PHASE-RELATED FEMTOSECOND PULSES

被引：30

作者：

WEFERS, MM

KAWASHIMA, H

NELSON, KA

机构：

[1] Department of Chemistry, Massachusetts Institute of Technology, Cambridge

来源：

JOURNAL OF CHEMICAL PHYSICS | 1995年 / 102卷 / 22期

关键词：

D O I：

10.1063/1.468862

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Multidimensional spectroscopy with femtosecond phase-related pulse sequences, in which the relative delays and optical phases of pulses are scanned during spectroscopic observation, is demonstrated on electronic transitions in atomic potassium vapor. The pulse sequences were constructed using emerging femtosecond pulse-shaping techniques that allow for automated generation of complex ultrafast waveforms. Sequences of two and three pulses with specified optical phase relationships and interpulse delays were used to prepare specified coherent states. © 1995 American Institute of Physics.

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页码：9133 / 9136

页数：4

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