DISPERSION-RELATION IN THE 3RD-ORDER ELECTRIC SUSCEPTIBILITY FOR POLYSILANE FILM

被引:36
作者
KISHIDA, H [1 ]
HASEGAWA, T [1 ]
IWASA, Y [1 ]
KODA, T [1 ]
TOKURA, Y [1 ]
机构
[1] UNIV TOKYO, DEPT PHYS, TOKYO 113, JAPAN
关键词
D O I
10.1103/PhysRevLett.70.3724
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The Kramers-Kronig (KK) dispersion relation has been proved to hold between independently measured spectra of the phase shift phi(omega) and the modulus \chi(3)(omega)\ of third-order electric susceptibility chi(3) (=\chi(3)\e(iphi)) for the third-order harmonic generation in silicon-based polymer poly(dihexylsilane) (PDHS) films, providing a direct experimental substantiation of the reciprocal KK relations in the non-linear optical solids. The reciprocal dispersion relations have been also found to hold for the real and imaginary parts of chi(3) in PDHS films.
引用
收藏
页码:3724 / 3727
页数:4
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