SURFACE-CHEMISTRY ON INTER-STELLAR OXIDE GRAINS

被引:7
作者
DENISON, P
WILLIAMS, DA
机构
[1] Mathematics Department, UMIST, PO Box 88, Manchester,M60 1QD, United Kingdom
关键词
Crystal surfaces - Diatomic molecules - Incident atoms - Interaction energies - Oxide grains - Perfect crystals - Surface vacancies - Vacancy sites - Williams;
D O I
10.1093/mnras/197.4.835
中图分类号
P1 [天文学];
学科分类号
0704 ;
摘要
Detailed calculations are made to test the predictions of Duley, Millar & Williams (1978) concerning the chemical reactivity of interstellar oxide grains. A method is established for calculating interaction energies between atoms and the perfect crystal with or without surface vacancy sites. The possibility of reactions between incident atoms and absorbed atoms is investigated. We conclude that H2 formation can occur on the perfect crystal surfaces, and that for other diatomic molecules the important formation sites are the Fs- and V22-centres. The outline by Duley, Millar & Williams (1979) of interstellar oxide grain growth and destruction is justified by these calculations. © 1981 Royal Astronomical Society.
引用
收藏
页码:835 / 844
页数:10
相关论文
共 19 条
[1]   DESTRUCTION AND GROWTH OF DUST GRAINS IN INTER-STELLAR SPACE .2. DESTRUCTION BY GRAIN SURFACE-REACTIONS, GRAIN-GRAIN COLLISIONS AND PHOTODESORPTION [J].
BARLOW, MJ .
MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY, 1978, 183 (02) :397-415
[2]   SHELL AND BREATHING SHELL-MODEL CALCULATIONS FOR DEFECT FORMATION ENERGIES AND VOLUMES IN MAGNESIUM-OXIDE [J].
CATLOW, CRA ;
FAUX, ID ;
NORGETT, MJ .
JOURNAL OF PHYSICS C-SOLID STATE PHYSICS, 1976, 9 (03) :419-429
[3]   POTENTIAL-ENERGY OF AN ISOLATED GOLD ATOM ON (100) SURFACE OF ALKALI-HALIDE CRYSTALS [J].
CHAN, EM ;
BUCKINGHAM, MJ ;
ROBINS, JL .
SURFACE SCIENCE, 1977, 67 (01) :285-298
[4]   INTERACTION POTENTIALS FOR ELASTIC-SCATTERING OF NOBLE-GAS ATOMS FROM CRYSTAL SURFACES [J].
DAVIES, RO ;
ULLERMAYER, LS .
SURFACE SCIENCE, 1973, 39 (01) :61-82
[5]   INFRARED STUDY OF INTERACTION OF HYDROGEN-SULFIDE AND WATER WITH A MAGNESIUM-OXIDE SURFACE [J].
DEANE, AM ;
GRIFFITHS, DL ;
LEWIS, IA ;
WINTER, JA ;
TENCH, AJ .
JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS I, 1975, 71 (05) :1005-1012
[6]   NEW MODEL FOR INTER-STELLAR DUST [J].
DULEY, WW ;
MILLAR, TJ ;
WILLIAMS, DA .
ASTROPHYSICS AND SPACE SCIENCE, 1979, 65 (01) :69-82
[7]  
DULEY WW, 1980, MON NOT R ASTRON SOC, V192, P945
[8]   MOLECULE PRODUCTION ON INTER-STELLAR OXIDE GRAINS [J].
DULEY, WW ;
MILLAR, TJ ;
WILLIAMS, DA .
MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY, 1978, 185 (03) :915-925
[9]   SCATTERING OF ATOMIC-HYDROGEN FROM MGO(001)-COVERED AND C2H5OH-COVERED LIF(001) SURFACES [J].
FRANK, H ;
HOINKES, H ;
WILSCH, H .
SURFACE SCIENCE, 1977, 62 (01) :326-330
[10]   MOLECULAR DIAGNOSTICS OF INTER-STELLAR SHOCKS [J].
HARTQUIST, TW ;
OPPENHEIMER, M ;
DALGARNO, A .
ASTROPHYSICAL JOURNAL, 1980, 236 (01) :182-188