THE DISTRIBUTION OF ARTIFICIAL RADIONUCLIDES IN THE ENGLISH-CHANNEL, SOUTHERN NORTH-SEA, SKAGERRAK AND KATTEGAT, 1990-1993

被引:42
作者
HERRMANN, J
KERSHAW, PJ
DUBOIS, PB
GUEGUENIAT, P
机构
[1] Bundesamt fur Seeschiffahrt und Hydrographie (BSH), D-20305 Hamburg
[2] Ministry of Agriculture, Fisheries and Food (MAFF), Directorate of Fisheries Research, Lowestoft
[3] Institut de Protection et de Sûreté Nucléaire (IPSN/CEA), Départment de Protection de l'Environnement et des Installations, Unité de Radioécologie Estuaires et Milieu Marin, Cedex
关键词
D O I
10.1016/0924-7963(95)00026-L
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
This paper presents the initial results concerning the distribution of artificial radionuclides from research cruises conducted in collaboration by three European institutes as part of an EEC MAST research project. Ten cruises were undertaken covering the English Channel, southern and eastern North Sea; Skagerrak and Kattegat over a period of 2.5 yr. A large number of analyses of four artificial radionuclides (Cs-137, Tc-99, Sb-125, Sr-90), which behave conservatively in seawater, provided information about the general distribution of water masses and circulation patterns as well as about single transport events in the study area. Controlled liquid releases from the La Hague nuclear fuel reprocessing plant are transported;eastwards, forming a characteristic distribution pattern in the Channel and the southern North Sea. This includes a near-coastal ''plume'' and a distinct boundary between waters contaminated predominantly by La Hague and by Sellafield. Spatial and temporal distributions of radionuclide ratios were used, for the first time, to calculate transit times from the English Channel to the coast of Jutland, The data published herein provide an essential input to the calibration of numerical models simulating water transport processes. The results demonstrate the continuing usefulness of artificial radionuclides as oceanographic tracers, even at the very low concentrations observed at present in north-west European Shelf waters.
引用
收藏
页码:427 / 456
页数:30
相关论文
共 27 条
[1]  
Aarkrog, Dahlgaard, Duniec, Guegueniat, Holm, The application of seaweeds as bioindicators for radioactive pollution in the Channel and southern North Sea, Radionuclides: a Tool for Oceanography, pp. 294-303, (1988)
[2]  
Bailly du Bois, Guegueniat, Gandon, Leon, Baron, Percentage contribution of inputs from the Atlantic, Irish Sea, English Channel and Baltic into the North Sea during 1988: a tracer-based evaluation using artificial radionuclides, Neth. J. Sea Res., 31, 1, pp. 1-10, (1993)
[3]  
Bailly du Bois, Salomon, Guegueniat, Gandon, A quantitative estimate of English Channel water fluxes into the North Sea from 1987 to 1992 based on radiotracer distribution, J. Mar. Syst., 6, pp. 457-481, (1995)
[4]  
Baker, The Determination of Radiocaesium in Sea and Fresh Waters, Fish. Res. Tech. Rep. MAFF, Direct. Fish. Res. Lowestoft, 16, (1975)
[5]  
Breton, Salomon, A 2D longterm advection-dispersion model for the Channel and southern North Sea. Part A: validation through comparison with artificial radionuclides, J. Mar. Syst., 6, pp. 495-513, (1995)
[6]  
Chen, Dahlgaard, Hansen, Aarkrog, Determination of <sup>99</sup>Tc in environmental samples by anion exchange and liquid-liquid extraction at controlled valency, Anal. Chim. Acta, 228, pp. 163-167, (1990)
[7]  
Dahlgaard, Chen, Herrmann, Nies, Ibbett, Kershaw, On the background level of <sup>99</sup>Tc, <sup>90</sup>Sr and <sup>137</sup>Cs in the North Atlantic, J. Mar. Syst., 6, pp. 571-578, (1995)
[8]  
Dahlgaard, Herrmann, Salomon, A tracer study of the transport of coastal water from the English Channel through the German Bight to the Kattegat, J. Mar. Syst., 6, pp. 415-425, (1995)
[9]  
Dahlgaard, Herrmann, van Weers, Masson, Ibbett, Chen, Quality assurance of the oceanographic tracers technetium-99 and antimony-125: intercomparisons and recovery tests, J. Mar. Syst., 6, pp. 391-396, (1995)
[10]  
Eicke, Gabriel, Wedekind, Verfahren zur Bestimmung von Strontium-90 im Meerwasser, Messanleitungen für die Überwachung der Radioaktivität in der Umwelt. Bundesminister des Inneren, Karlsruhe, (1984)