ANTIFERROMAGNETIC LONG-RANGE ORDER CAUSED BY NONMAGNETIC IMPURITIES - MAGNETIZATION OF SINGLE-CRYSTAL CU1-XZNXGEO3

被引:105
作者
HASE, M [1 ]
KOIDE, N [1 ]
MANABE, K [1 ]
SASAGO, Y [1 ]
UCHINOKURA, K [1 ]
SAWA, A [1 ]
机构
[1] ELECTROTECH LAB,TSUKUBA,IBARAKI 305,JAPAN
来源
PHYSICA B | 1995年 / 215卷 / 2-3期
关键词
D O I
10.1016/0921-4526(95)00405-X
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
The magnetization was obtained as a function of temperature and magnetic field of a Cu1-xZnxGeO3 single-crystal with x similar to 0.04. The temperature dependence of the magnetic susceptibility in 0.1 T parallel to the c axis shows a clear cusp around 4.5 K and decreases rapidly below 4.5 K. There is no hysteresis between the data measured in zero-field-cooling and held-cooling processes, The field dependence of the magnetization parallel to the c axis at 2.0 K exhibits an apparent increase around 1.OT, which corresponds to a spin-flop transition. The temperature and held dependences, the anisotropy, and the absence of the hysteresis undoubtedly prove the occurrence of an antiferromagnetic long-range order below 4.5 K instead of the spin-glass-like transition reported previously. Spins below the transition temperature are ordered almost parallel to the c axis. This is the first report of magnetic long-range order caused by nonmagnetic impurities.
引用
收藏
页码:164 / 170
页数:7
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