IRREVERSIBLE ADSORPTION ON NONUNIFORM SURFACES - THE RANDOM SITE MODEL

被引:65
作者
JIN, XZ
WANG, NHL
TARJUS, G
TALBOT, J
机构
[1] PURDUE UNIV,SCH CHEM ENGN,W LAFAYETTE,IN 47907
[2] UNIV PARIS 06,PHYS THEOR LIQUIDES,F-75252 PARIS 05,FRANCE
关键词
D O I
10.1021/j100119a003
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The random sequential adsorption (RSA) process provides a starting point for the development of quantitative descriptions of the irreversible adsorption of proteins and other large molecules. To date, none of the numerous theoretical and computational studies of RSA have considered the effect of nonuniform aperiodic substrates which are present in many physical systems. We study the irreversible adsorption of spherical particles adsorbing on randomly distributed point sites. There exists an unexpected, yet simple, mapping between this process and the corresponding adsorption on a smooth, continuous surface.
引用
收藏
页码:4256 / 4258
页数:3
相关论文
共 12 条
[1]  
CHASE HA, 1984, CHEM ENG SCI, V39, P1099
[2]   SELECTIVE ENZYME PURIFICATION BY AFFINITY CHROMATOGRAPHY [J].
CUATRECA.P ;
WILCHEK, M ;
ANFINSEN, CB .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 1968, 61 (02) :636-&
[3]   RANDOM SEQUENTIAL ADSORPTION [J].
FEDER, J .
JOURNAL OF THEORETICAL BIOLOGY, 1980, 87 (02) :237-254
[4]   LIQUID-STATE METHODS FOR RANDOM-MEDIA - RANDOM SEQUENTIAL ADSORPTION [J].
GIVEN, JA .
PHYSICAL REVIEW A, 1992, 45 (02) :816-824
[5]  
GONZALEZ JJ, 1974, CHEM PHYS, V3, P288
[6]  
MEAKIN P, IN PRESS PHYS REV A
[7]   EXPERIMENTAL-DETERMINATION OF THE RANDOM-PARKING LIMIT IN 2 DIMENSIONS [J].
ONODA, GY ;
LINIGER, EG .
PHYSICAL REVIEW A, 1986, 33 (01) :715-716
[8]   SURFACE EXCLUSION EFFECTS IN ADSORPTION PROCESSES [J].
SCHAAF, P ;
TALBOT, J .
JOURNAL OF CHEMICAL PHYSICS, 1989, 91 (07) :4401-4409
[9]   PROPERTIES OF JAMMING CONFIGURATIONS BUILT UP BY THE ADSORPTION OF BROWNIAN PARTICLES ONTO SOLID-SURFACES [J].
SENGER, B ;
VOEGEL, JC ;
SCHAAF, P ;
JOHNER, A ;
SCHMITT, A ;
TALBOT, J .
PHYSICAL REVIEW A, 1991, 44 (10) :6926-6928
[10]   UNEXPECTED ASYMPTOTIC-BEHAVIOR IN RANDOM SEQUENTIAL ADSORPTION OF NONSPHERICAL PARTICLES [J].
TALBOT, J ;
TARJUS, G ;
SCHAAF, P .
PHYSICAL REVIEW A, 1989, 40 (08) :4808-4811