QUENCHING OF 2-PHOTON FLUORESCENCE AND STIMULATED ANTI-STOKES EMISSION IN RHODAMINE SOLUTIONS

被引:1
作者
EICHLER, HJ
LANGHANS, D
KLEIN, U
机构
[1] Universität Berlin, Optisches Institut, Berlin 12
关键词
D O I
10.1364/AO.18.001383
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Two-photon fluorescence (TPF) has been excited in different solutions of rhodamine 6G and rhodamine B with single 30-psec pulses from a Nd:YAG laser at 1.06 μm.Up to incident intensities of 6 × 1028 photons cm−2 sec−1 the TPF intensity showed a quadratic dependence on the photon flux.At higher photon fluxes the TPF intensity increased less than quadratically with the incident intensity.A possible mechanism, not considered previously, for this quenching is stimulated Raman scattering.It was observed that TPF-quenching and stimulated anti-Stokes emission had thresholds in the same power range.© 1979 Optical Society of America.
引用
收藏
页码:1383 / 1386
页数:4
相关论文
共 8 条
[1]   INTERACTIONS OF PICOSECOND LASER PULSES WITH ORGANIC-MOLECULES .1. 2-PHOTON FLUORESCENCE QUENCHING AND SINGLET STATES EXCITATION IN RHODAMINE DYES [J].
BRADLEY, DJ ;
NEW, GHC ;
PETTY, MS ;
HUTCHINS.MH ;
MORROW, T ;
KOETSER, H .
PROCEEDINGS OF THE ROYAL SOCIETY OF LONDON SERIES A-MATHEMATICAL AND PHYSICAL SCIENCES, 1972, 328 (1572) :97-+
[2]   INTERACTIONS OF PICOSECOND LASER PULSES WITH ORGANIC-MOLECULES .2. 2-PHOTON ABSORPTION CROSS-SECTIONS [J].
BRADLEY, DJ ;
KOETSER, H ;
HUTCHINSON, MH .
PROCEEDINGS OF THE ROYAL SOCIETY OF LONDON SERIES A-MATHEMATICAL AND PHYSICAL SCIENCES, 1972, 329 (1576) :105-+
[3]   2-PHOTON EXCITATION OF FLUORESCENCE BY PICOSECOND LIGHT PULSES [J].
GIORDMAINE, JA ;
RENTZEPIS, PM ;
SHAPIRO, SL ;
WECHT, KW .
APPLIED PHYSICS LETTERS, 1967, 11 (07) :216-+
[4]   PICOSECOND SPECTROSCOPY OF MOLECULAR VIBRATIONS IN LIQUIDS - VIBRATIONAL BOTTLENECK IN ETHANOL [J].
LAUBEREAU, A ;
KEHL, G ;
KAISER, W .
OPTICS COMMUNICATIONS, 1974, 11 (01) :74-77
[5]  
Mory S., 1972, Optics Communications, V6, P394, DOI 10.1016/0030-4018(72)90165-4
[6]  
Rapp W, 1971, CHEM PHYS LETT, V8, P529, DOI 10.1016/0009-2614(71)80084-2
[7]  
VONDERLINDE D, 1972, IEEE J QUANTUM ELECT, V8, P328