LAMELLAR PEROVSKITES BI2O2(AN-1BNO3N+1) CATALYSTS FOR OXIDATIVE COUPLING OF METHANE

被引:9
作者
BARRAULT, J [1 ]
GROSSET, C [1 ]
DION, M [1 ]
GANNE, M [1 ]
TOURNOUX, M [1 ]
机构
[1] INST MAT NANTES,CHIM SOLIDES LAB,F-44072 NANTES 03,FRANCE
关键词
METHANE; OXIDATIVE COUPLING; LAMELLAR PEROVSKITES; AURIVILLIUS PHASES;
D O I
10.1007/BF00764372
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The oxidative coupling of methane has been studied in the presence of lamellar perovskites Bi2O2(An-1BnO3n+1) belonging to Aurivillius phases. These materials are selective and stable in the OCM reaction. Moreover, their substitution in perovskite (A) or octahedral (B) sites leads to significant changes of the C2+ selectivity or yield which are attributed to modifications of the basicity of A-O or B-O bonds.
引用
收藏
页码:203 / 210
页数:8
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