AUGER AND PHOTOELECTRON STUDY OF THE HUBBARD-U IN C-60, K3C60, AND K6C60

被引:72
作者
BRUHWILER, PA [1 ]
MAXWELL, AJ [1 ]
NILSSON, A [1 ]
MARTENSSON, N [1 ]
GUNNARSSON, O [1 ]
机构
[1] MAX PLANCK INST FESTKORPERFORSCH,D-70569 STUTTGART 80,GERMANY
来源
PHYSICAL REVIEW B | 1993年 / 48卷 / 24期
关键词
D O I
10.1103/PhysRevB.48.18296
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Comparison of valence-photoelectron to Auger-electron spectra has been carried out fbr three phases of KxC60, x = 0, 3, 6, yielding Hubbard correlation energies, U, of 1.4 eV (1.5 eV) for x =0 (6), consistent with the results of Lof et al. [Phys. Rev. Lett. 68, 3924 (1992)]. At x = 3 the results are best described by intermolecular charge-transfer screening of the C Is core hole in the Auger initial state, with U of the same magnitude as for x = 0 and 6.
引用
收藏
页码:18296 / 18299
页数:4
相关论文
共 37 条
  • [1] CHARACTERIZATION OF THE SOLUBLE ALL-CARBON MOLECULES C60 AND C70
    AJIE, H
    ALVAREZ, MM
    ANZ, SJ
    BECK, RD
    DIEDERICH, F
    FOSTIROPOULOS, K
    HUFFMAN, DR
    KRATSCHMER, W
    RUBIN, Y
    SCHRIVER, KE
    SENSHARMA, D
    WHETTEN, RL
    [J]. JOURNAL OF PHYSICAL CHEMISTRY, 1990, 94 (24) : 8630 - 8633
  • [2] ANDERSEN JN, 1991, SYNCHROTRON RAD NEWS, V4, P15
  • [3] COULOMB INTEGRALS AND MODEL HAMILTONIANS FOR C-60
    ANTROPOV, VP
    GUNNARSSON, O
    JEPSEN, O
    [J]. PHYSICAL REVIEW B, 1992, 46 (20): : 13647 - 13650
  • [4] C-60 AND C-70 FULLERENES AND POTASSIUM FULLERIDES
    BENNING, PJ
    POIRIER, DM
    OHNO, TR
    CHEN, Y
    JOST, MB
    STEPNIAK, F
    KROLL, GH
    WEAVER, JH
    FURE, J
    SMALLEY, RE
    [J]. PHYSICAL REVIEW B, 1992, 45 (12): : 6899 - 6913
  • [5] DETERMINATION OF TIME SCALES FOR CHARGE-TRANSFER SCREENING IN PHYSISORBED MOLECULES
    BJORNEHOLM, O
    NILSSON, A
    SANDELL, A
    HERNNAS, B
    MARTENSSON, N
    [J]. PHYSICAL REVIEW LETTERS, 1992, 68 (12) : 1892 - 1895
  • [6] AUTOIONIZATION AND AUGER-SPECTRA OF C-60 FILMS - IMPLICATIONS FOR CHARGE SCREENING AND TRANSPORT
    BRUHWILER, PA
    MAXWELL, AJ
    MARTENSSON, N
    [J]. INTERNATIONAL JOURNAL OF MODERN PHYSICS B, 1992, 6 (23-24): : 3923 - 3929
  • [7] BRUHWILER PA, UNPUB
  • [8] BRUHWILER PA, IN PRESS PHYS REV LE
  • [9] ELECTRONIC STATES AND PHASES OF KXC60 FROM PHOTOEMISSION AND X-RAY ABSORPTION-SPECTROSCOPY
    CHEN, CT
    TJENG, LH
    RUDOLF, P
    MEIGS, G
    ROWE, JE
    CHEN, J
    MCCAULEY, JP
    SMITH, AB
    MCGHIE, AR
    ROMANOW, WJ
    PLUMMER, EW
    [J]. NATURE, 1991, 352 (6336) : 603 - 605
  • [10] MANY-BODY PROCESSES IN X-RAY PHOTOEMISSION LINE-SHAPES FROM LI, NA, MG, AND AL METALS
    CITRIN, PH
    WERTHEIM, GK
    BAER, Y
    [J]. PHYSICAL REVIEW B, 1977, 16 (10) : 4256 - 4282