NEUTRON AND LIGHT-SCATTERING STUDY OF SUPERCOOLED GLYCEROL

被引:205
作者
WUTTKE, J
HERNANDEZ, J
LI, G
CODDENS, G
CUMMINS, HZ
FUJARA, F
PETRY, W
SILLESCU, H
机构
[1] UNIV MAINZ,INST PHYS CHEM,D-55128 MAINZ,GERMANY
[2] CUNY CITY COLL,NEW YORK,NY 10031
[3] CENS,LAB LEON BRILLOVIN,F-91191 GIF SUR YVETTE,FRANCE
关键词
D O I
10.1103/PhysRevLett.72.3052
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Relaxation dynamics was investigated in the hydrogen-bonded glass former glycerol using incoherent neutron scattering and depolarized light scattering. The neutron data have a q-independent form in the intermediate beta-relaxation regime implying factorization of the q and omega dependences. Similar susceptibility spectra were obtained from both data sets qualitatively resembling the mode coupling theory scenario. Quantitative fits indicate apparent deviations of the exponents from mode coupling theory predictions suggesting that the influence of vibrational modes is severe in network glass formers.
引用
收藏
页码:3052 / 3055
页数:4
相关论文
共 28 条
[1]  
ANDRUSSOW L, 1969, LANDOLTBORNSTEIN 5A, V2
[2]   THERMODYNAMICS OF GLASS-TRANSITION - EMPIRICAL ASPECTS [J].
ANGELL, CA ;
SICHINA, W .
ANNALS OF THE NEW YORK ACADEMY OF SCIENCES, 1976, 279 (OCT15) :53-67
[3]   SPECIFIC-HEAT SPECTROSCOPY OF THE GLASS-TRANSITION [J].
BIRGE, NO ;
NAGEL, SR .
PHYSICAL REVIEW LETTERS, 1985, 54 (25) :2674-2677
[4]   MEASUREMENT OF QUASI-ELASTIC LINE-BROADENING IN GLYCEROL WITH A NEUTRON CRYSTAL SPECTROMETER OF EXTREMELY HIGH ENERGY RESOLUTION [J].
BIRR, M .
ZEITSCHRIFT FUR PHYSIK, 1970, 238 (03) :221-&
[5]   LIGHT-SCATTERING SPECTROSCOPY OF THE LIQUID-GLASS TRANSITION IN CAKNO3 AND IN THE MOLECULAR GLASS SALOL - EXTENDED-MODE-COUPLING-THEORY ANALYSIS [J].
CUMMINS, HZ ;
DU, WM ;
FUCHS, M ;
GOTZE, W ;
HILDEBRAND, S ;
LATZ, A ;
LI, G ;
TAO, NJ .
PHYSICAL REVIEW E, 1993, 47 (06) :4223-4239
[6]   DIELECTRIC RELAXATION IN GLYCEROL, PROPYLENE GLYCOL, AND NORMAL-PROPANOL [J].
DAVIDSON, DW ;
COLE, RH .
JOURNAL OF CHEMICAL PHYSICS, 1951, 19 (12) :1484-1490
[7]   REORIENTATION IN ASSOCIATED LIQUIDS .1. GLYCEROL [J].
DUX, H ;
DORFMULLER, T .
CHEMICAL PHYSICS, 1979, 40 (1-2) :219-227
[8]   MOLECULAR-MOTION IN SUPERCOOLED GLYCEROL .2. TEMPERATURE-DEPENDENCE FROM MOSSBAUER SCATTERING [J].
ELWENSPOEK, M ;
SOLTWISCH, M ;
QUITMANN, D .
MOLECULAR PHYSICS, 1978, 35 (05) :1221-1231
[9]   STUDY OF THE GLASS-TRANSITION ORDER PARAMETER IN AMORPHOUS POLYBUTADIENE BY INCOHERENT NEUTRON-SCATTERING [J].
FRICK, B ;
RICHTER, D ;
PETRY, W ;
BUCHENAU, U .
ZEITSCHRIFT FUR PHYSIK B-CONDENSED MATTER, 1988, 70 (01) :73-79
[10]   LOCALIZED MOTION IN SUPERCOOLED GLYCEROL AS MEASURED BY H-2-NMR SPIN-LATTICE RELAXATION AND INCOHERENT NEUTRON-SCATTERING [J].
FUJARA, F ;
PETRY, W ;
DIEHL, RM ;
SCHNAUSS, W ;
SILLESCU, H .
EUROPHYSICS LETTERS, 1991, 14 (06) :563-568