SURFACE LAYERING IN LIQUID GALLIUM - AN X-RAY REFLECTIVITY STUDY

被引:270
作者
REGAN, MJ
KAWAMOTO, EH
LEE, S
PERSHAN, PS
MASKIL, N
DEUTSCH, M
MAGNUSSEN, OM
OCKO, BM
BERMAN, LE
机构
[1] HARVARD UNIV, DIV APPL SCI, CAMBRIDGE, MA 02138 USA
[2] HARVARD UNIV, DEPT PHYS, CAMBRIDGE, MA 02138 USA
[3] BAR ILAN UNIV, DEPT PHYS, IL-52100 RAMAT GAN, ISRAEL
[4] BROOKHAVEN NATL LAB, DEPT PHYS, UPTON, NY 11973 USA
[5] BROOKHAVEN NATL LAB, NATL SYNCHROTRON LIGHT SOURCE, UPTON, NY 11973 USA
关键词
D O I
10.1103/PhysRevLett.75.2498
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Surface-induced atomic layering in liquid gallium has been observed using x-ray reflectivity, ultrahigh vacuum conditions, and sputtered clean surfaces. Reflectivity data, collected on a supercooled liquid sample to momentum transfers as large as q(z) = 3.0 Angstrom(-1), exhibit a strong maximum near 2.4 Angstrom(-1) indicating a layer spacing that is comparable to its atomic dimensions. The amplitude of the electron density oscillations decays with a characteristic length of 6 Angstrom. This is unexpectedly twice that of recent results for Hg, and the difference may be related to covalent bonding or supercooling.
引用
收藏
页码:2498 / 2501
页数:4
相关论文
共 26 条
  • [1] ATOMIC RADIAL DISTRIBUTIONS AND ION-ION POTENTIAL IN LIQUID GALLIUM
    ASCARELLI, P
    [J]. PHYSICAL REVIEW, 1966, 143 (01): : 36 - +
  • [2] INSITU STUDIES OF ELECTROCHEMICAL INTERFACES BY GRAZING ANGLE X-RAY REFLECTION
    BOSIO, L
    CORTES, R
    FOLCHER, G
    FROMENT, M
    [J]. JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1992, 139 (08) : 2110 - 2114
  • [3] CAPILLARY WAVES ON THE SURFACE OF SIMPLE LIQUIDS MEASURED BY X-RAY REFLECTIVITY
    BRASLAU, A
    PERSHAN, PS
    SWISLOW, G
    OCKO, BM
    ALSNIELSEN, J
    [J]. PHYSICAL REVIEW A, 1988, 38 (05): : 2457 - 2470
  • [4] CAI ZH, UNPUB
  • [5] A STUDY OF THE LIQUID-VAPOR INTERFACE OF MERCURY - COMPUTER-SIMULATION RESULTS
    DEVELYN, MP
    RICE, SA
    [J]. JOURNAL OF CHEMICAL PHYSICS, 1983, 78 (08) : 5081 - 5095
  • [6] DICICCO A, 1994, EUROPHYS LETT, V27, P407, DOI 10.1209/0295-5075/27/5/013
  • [7] EVANS R, 1980, J PHYSIQUE, V41, P775
  • [8] INPLANE STRUCTURE OF THE LIQUID-VAPOR INTERFACE OF AN ALLOY - A GRAZING-INCIDENCE X-RAY-DIFFRACTION STUDY OF BISMUTH GALLIUM
    FLOM, EB
    LI, MY
    ACERO, A
    MASKIL, N
    RICE, SA
    [J]. SCIENCE, 1993, 260 (5106) : 332 - 335
  • [9] A GRAZING-INCIDENCE X-RAY-DIFFRACTION STUDY OF THE TRANSVERSE STRUCTURE-FUNCTION OF THE LIQUID-VAPOR INTERFACE OF GA
    FLOM, EB
    CAI, ZH
    ACERO, A
    LIN, BH
    MASKIL, N
    LIU, L
    RICE, SA
    [J]. JOURNAL OF CHEMICAL PHYSICS, 1992, 96 (06) : 4743 - 4749
  • [10] STRUCTURE AND SURFACE-TENSION OF THE LIQUID-VAPOR INTERFACE OF SIMPLE METALS - A THEORETICAL APPROACH
    GOMEZ, MA
    CHACON, E
    [J]. PHYSICAL REVIEW B, 1992, 46 (02): : 723 - 732