UNIFIED DESCRIPTION OF ROTATING-MOLECULE SURFACE INTERACTIONS - COMPARISON WITH EXPERIMENT

被引:17
作者
HOOGEVEEN, RWM [1 ]
HERMANS, LJF [1 ]
BORMAN, VD [1 ]
KRYLOV, SY [1 ]
机构
[1] MOSCOW ENGN PHYS INST, MOSCOW, USSR
关键词
D O I
10.1103/PhysRevA.42.6480
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
From previous experiments on surface light-induced drift it was found that the coefficient for tangential momentum accommodation in molecule-surface collisions can increase with increasing angular momentum of the molecule. By contrast, various molecular-beam-type experiments yielded the opposite result. These seemingly conflicting data are reconciled in a unified picture describing various phenomena related to molecule-surface interaction for rotating molecules. Using physical arguments it is demonstrated that the accommodation as a function of rotational quantum number should peak around the thermal value, decreasing both for lower and higher rotational quantum numbers of the incoming molecule. © 1990 The American Physical Society.
引用
收藏
页码:6480 / 6485
页数:6
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