THE GLASS-TRANSITION IN (KI)0.5(ND4I)0.5 MIXED-CRYSTALS AS STUDIED BY DEUTERON SPIN-LATTICE RELAXATION

被引:15
作者
BOHMER, R [1 ]
FUJARA, F [1 ]
HINZE, G [1 ]
机构
[1] UNIV MAINZ,INST PHYS CHEM,W-6500 MAINZ,GERMANY
关键词
D O I
10.1016/0038-1098(93)90898-W
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
Nuclear spin resonance has been used to study the deuteron magnetization recovery in (KI)0.5(ND4I)0.5 mixed crystals. At high temperatures the spin-lattice-relaxation is exponential. For T less than or similar to 45 K deviations from this simple behaviour occur, signalling the onset of spatial inhomogeneities due to the formation of an orientational glass. The results demonstrate that the transition of (KI)0.5(ND4I)0.5 into the glassy state is driven by the freezing of random bonds.
引用
收藏
页码:183 / 186
页数:4
相关论文
共 24 条
[1]   GLASSLIKE THERMAL-PROPERTIES AND ISOTOPE EFFECT IN RB1-X(NH4)XH2PO4 MIXED-CRYSTALS [J].
BERRET, JF ;
MEISSNER, M ;
WATSON, SK ;
POHL, RO ;
COURTENS, E .
PHYSICAL REVIEW LETTERS, 1991, 67 (01) :93-96
[2]   RAMAN INVESTIGATION OF ROTATIONAL AND TRANSLATIONAL EXCITATIONS IN K1-X(NH4)XI MIXED-CRYSTALS [J].
BERRET, JF ;
SAUVAJOL, JL ;
HAUSSUHL, S .
JOURNAL OF CHEMICAL PHYSICS, 1992, 96 (07) :4896-4903
[3]   ANOMALOUS THERMOELASTIC BEHAVIOR OF (KI)1-X(NH4I)X [J].
BERRET, JF ;
BRUCHHAUSER, F ;
FEILE, R ;
BOSTOEN, C ;
HAUSSUHL, S .
SOLID STATE COMMUNICATIONS, 1990, 74 (10) :1041-1045
[4]   PHONON SOFTENING, ORIENTATIONAL SLOWING-DOWN AND DIFFUSE-SCATTERING IN (KI)1-X(ND4I)X MIXED-CRYSTALS [J].
BERRET, JF ;
BOSTOEN, C ;
SAUVAJOL, JL ;
HENNION, B ;
HAUSSUHL, S .
EUROPHYSICS LETTERS, 1991, 16 (01) :91-96
[5]   THEORY OF ORIENTATIONAL GLASSES MODELS, CONCEPTS, SIMULATIONS [J].
BINDER, K ;
REGER, JD .
ADVANCES IN PHYSICS, 1992, 41 (06) :547-627
[6]   ND4 DEUTERON NMR AND THE SMEARING OF THE GLASS-TRANSITION IN RB1-X(ND4)XD2PO4 [J].
BLINC, R ;
DOLINSEK, J ;
SCHMIDT, VH ;
AILION, DC .
EUROPHYSICS LETTERS, 1988, 6 (01) :55-60
[7]   LOCAL-POLARIZATION DISTRIBUTION IN DEUTERON GLASSES [J].
BLINC, R ;
DOLINSEK, J ;
PIRC, R ;
TADIC, B ;
ZALAR, B ;
KIND, R ;
LIECHTI, O .
PHYSICAL REVIEW LETTERS, 1989, 63 (20) :2248-2251
[8]  
BLINC R, 1986, PHYS REV LETT, V57, P2926
[9]   ROTATIONAL EXCITATIONS IN K1-X(NH4)XI MIXED-CRYSTALS - A NEUTRON-SCATTERING STUDY [J].
BOSTOEN, C ;
CODDENS, G ;
WEGENER, W .
JOURNAL OF CHEMICAL PHYSICS, 1989, 91 (10) :6337-6344
[10]   LOW-ENERGY EXCITATIONS IN (KBR)1-X(KCN)X IN THE ORIENTATIONAL GLASS STATE [J].
DEYOREO, JJ ;
MEISSNER, M ;
POHL, RO ;
ROWE, JM ;
RUSH, JJ ;
SUSMAN, S .
PHYSICAL REVIEW LETTERS, 1983, 51 (12) :1050-1053