STOICHIOMETRIC PHOTOCATALYTIC DECOMPOSITION OF PURE WATER IN PT/TIO2 AQUEOUS SUSPENSION SYSTEM

被引:127
作者
TABATA, S
NISHIDA, H
MASAKI, Y
TABATA, K
机构
[1] Research Institute of Innovative Technology for the Earth (RITE), Kyoto, 619-02, Kizugawadai 9-2, Kizucho
关键词
PHOTOCATALYSIS; WATER DECOMPOSITION; PT/TIO2; SUSPENSION;
D O I
10.1007/BF00808339
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The influence of the direction of ultraviolet irradiation upon the yields of the photocatalytic decomposition of pure water has been investigated in Pt/TiO2 aqueous suspension system. The yields of the photocatalytic decomposition irradiated from the top of the reaction cell are about 10(3) times higher than those irradiated from the bottom. The difference seems due to the reverse reaction of the formed H-2 and O-2 in the suspension.
引用
收藏
页码:245 / 249
页数:5
相关论文
共 10 条
[1]   DYNAMICS OF LIGHT-INDUCED WATER CLEAVAGE IN COLLOIDAL SYSTEMS [J].
DUONGHONG, D ;
BORGARELLO, E ;
GRATZEL, M .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1981, 103 (16) :4685-4690
[2]   PHOTOCATALYTIC DECOMPOSITION OF GASEOUS WATER OVER TIO2 AND TIO2-RUO2 SURFACES [J].
KAWAI, T ;
SAKATA, T .
CHEMICAL PHYSICS LETTERS, 1980, 72 (01) :87-89
[3]   PHOTOCATALYTIC ACTIVITIES OF TIO2 LOADED WITH NIO [J].
KUDO, A ;
DOMEN, K ;
MARUYA, K ;
ONISHI, T .
CHEMICAL PHYSICS LETTERS, 1987, 133 (06) :517-519
[4]   HYDROGEN AND OXYGEN PHOTOPRODUCTION BY TITANATE POWDERS [J].
MAGLIOZZO, RS ;
KRASNA, AI .
PHOTOCHEMISTRY AND PHOTOBIOLOGY, 1983, 38 (01) :15-21
[5]   PHOTOSENSITIZED DISSOCIATION OF WATER USING DISPERSED SUSPENSIONS OF N-TYPE SEMICONDUCTORS [J].
MILLS, A ;
PORTER, G .
JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS I, 1982, 78 :3659-3669
[6]   SPECTROSCOPIC CHARACTERIZATION AND PHOTOCHEMICAL BEHAVIOR OF A TITANIUM HYDROXYPEROXO COMPOUND [J].
MUNUERA, G ;
GONZALEZELIPE, AR ;
FERNANDEZ, A ;
MALET, P ;
ESPINOS, JP .
JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS I, 1989, 85 :1279-1290
[7]  
SAKATA Y, 1993, CHEM LETT, P2381
[8]   PHOTO-DECOMPOSITION OF WATER OVER P-TIO2 CATALYSTS [J].
SATO, S ;
WHITE, JM .
CHEMICAL PHYSICS LETTERS, 1980, 72 (01) :83-86
[9]  
SATO S, 1988, NEW J CHEM, V12, P859
[10]   EFFECT OF NA2CO3 ADDITION ON PHOTOCATALYTIC DECOMPOSITION OF LIQUID WATER OVER VARIOUS SEMICONDUCTOR CATALYSTS [J].
SAYAMA, K ;
ARAKAWA, H .
JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY, 1994, 77 (2-3) :243-247