NEPTUNIUM IN INTERTIDAL COASTAL AND ESTUARINE SEDIMENTS IN THE IRISH SEA

被引:16
作者
ASSINDER, DJ
YAMAMOTO, M
KIM, CK
SEKI, R
TAKAKU, Y
YAMAUCHI, Y
KOMURA, K
UENO, K
BOURNE, GS
机构
[1] Low Level Radioactivity Laboratory, Kanazawa University, Tatsunokuchi, Ishikawa
[2] Department of Chemistry, University of Tsukuba, Tsukuba, Ibaraki
[3] Marubun Co., Tokyo, 103, 8-1 Odenma-cho, Nihonbashi
关键词
D O I
10.1016/0265-931X(91)90073-O
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A survey has been carried out of Np-237 activities in sediments of the Irish Sea. Two independent methods of analysis were used (ICP-MS and alpha-spectrometry) to enable the intercomparison of the results produced. The Np-237 content of the samples ranged from 0.01-4.5 Bq/kg for all areas apart from the Ribble Estuary. In the Ribble, a source of Np-237 other than Sellafield has been found which supports Np-237 activities in sediments up to 13.3 Bq/kg. This anomaly is verified by comparing Np-237 with the Pu-239, Pu-240 content of the sediments. These are believed to be the highest environmental Np-237 values yet recorded.
引用
收藏
页码:135 / 145
页数:11
相关论文
共 17 条
[1]  
Allard, Solubilities of actinides in neutral or basic solutions, Actinides in Perspective, (1982)
[2]  
Aston, Assinder, Kelly, Plutonium in intertidal coastal and estuarine sediments in the northern Irish Sea, Est. Coastal and Shelf Sci., 20, pp. 761-771, (1985)
[3]  
BNFL, Annual report on radioactive discharges and monitoring of the environment, 1979–1988, (1980)
[4]  
Bondietti, Tamura, Physico-chemical associations of plutonium and other actinides in soil, Transuranic Elements in the Environment, pp. 145-164, (1980)
[5]  
Byrne, Determination of <sup>237</sup>Np in Cumbrian sediments by neutron activation analysis: preliminary results, J. Environ. Radioactivity, 4, pp. 133-144, (1986)
[6]  
Cohen, Effects of ICRP Publication 30 and the 1980 BEIR report on hazard assessments of high-level waste, Health Physics, 42, pp. 133-143, (1982)
[7]  
Edgington, Nelson, The chemical behaviour of long-lived radionuclides in the marine environment, International Symposium on the Behaviour of Long-Lived Radionuclides in the Marine Environment, pp. 19-66, (1984)
[8]  
Germain, Gandon, Masson, Guegueniat, Experimental studies of the transfer of neptunium from sea water to sediments and organisms (annelids and molluscs), J. Environ. Radioactivity, 5, pp. 37-55, (1987)
[9]  
Harvey, Potential for post-depositional migration of neptunium in Irish Sea sediments, Impacts of Radionuclide Release in the Marine Environment, pp. 93-103, (1981)
[10]  
Harvey, Kershaw, Physico-chemical interactions of long-lived radionuclides in coastal marine sediments and some comparisons with deep sea environments, Eur. Rep. Comm. Eur. Commun., EUR-9214, (1984)