EXCITATION WITHOUT DEMOLITION - RADIATIVE EXCITATION OF GROUND-SURFACE VIBRATION BY IMPULSIVE STIMULATED RAMAN-SCATTERING WITH DAMAGE CONTROL

被引:122
作者
KOSLOFF, R
DELLHAMMERICH, A
TANNOR, D
机构
[1] HEBREW UNIV JERUSALEM,FRITZ HABER RES CTR,IL-91904 JERUSALEM,ISRAEL
[2] UNIV NOTRE DAME,DEPT CHEM & BIOCHEM,NOTRE DAME,IN 46556
关键词
D O I
10.1103/PhysRevLett.69.2172
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
A pulse shaping strategy is developed for exciting the ground-surface vibrational motion while minimizing radiation damage. The scheme is based on a resonant impulsive stimulated Raman scattering process where the amount of population transferred to the excited surface is strictly controlled. The scenario begins with an impulsive pulse which creates an instantaneous dipole moment. It follows by a pulse 180-degrees out of phase with the instantaneous dipole which deposits vibrational energy into the ground electronic surface while blocking population transfer to the excited surface.
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页码:2172 / 2175
页数:4
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