HOLE BURNING OF LONG-CHAIN MOLECULAR AGGREGATES - HOMOGENEOUS LINE BROADENING, SPECTRAL-DIFFUSION BROADENING, AND PRESSURE BROADENING

被引:14
作者
HIRSCHMANN, R [1 ]
FRIEDRICH, J [1 ]
机构
[1] UNIV BAYREUTH,BAYREUTHER INST MAKROMOLEK FORSCH,W-8580 BAYREUTH,GERMANY
关键词
D O I
10.1364/JOSAB.9.000811
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We investigate broadening phenomena of spectral holes burned into delocalized states of molecular aggregates. We measured spectral-diffusion broadening, homogeneous line broadening, and pressure-induced line broadening. The behavior is quite different from that for localized states. Whereas homogeneous broadening is dominated by exciton-phonon scattering, spectral-diffusion broadening and pressure broadening are extremely small because of large motional narrowing effects.
引用
收藏
页码:811 / 815
页数:5
相关论文
共 33 条
[1]   DYNAMICS IN LOW-TEMPERATURE GLASSES - THEORY AND EXPERIMENTS ON OPTICAL DEPHASING, SPECTRAL DIFFUSION, AND HYDROGEN TUNNELING [J].
BERG, M ;
WALSH, CA ;
NARASIMHAN, LR ;
LITTAU, KA ;
FAYER, MD .
JOURNAL OF CHEMICAL PHYSICS, 1988, 88 (03) :1564-1587
[2]  
BREINL W, 1984, J CHEM PHYS, V81, P3916
[3]  
BURLAND D, 1977, J CHEM PHYS, V67, P1929
[4]  
DALTROZZO E, 1974, PHOTOGR SCI ENG, V18, P441
[5]   DEPHASING-INDUCED DAMPING OF SUPERRADIANT EMISSION IN J-AGGREGATES [J].
DEBOER, S ;
WIERSMA, DA .
CHEMICAL PHYSICS LETTERS, 1990, 165 (01) :45-53
[6]   OPTICAL-DYNAMICS OF EXCITON AND POLARON FORMATION IN MOLECULAR AGGREGATES [J].
DEBOER, S ;
WIERSMA, DA .
CHEMICAL PHYSICS, 1989, 131 (01) :135-144
[7]  
DEBOER S, 1987, CHEM PHYS LETT, V137, P91
[8]   COHERENT ENERGY MIGRATION IN SOLIDS .1. BAND-TRAP EQUILIBRIA AT BOLTZMANN AND NONBOLTZMANN TEMPERATURES [J].
FAYER, MD ;
HARRIS, CB .
PHYSICAL REVIEW B, 1974, 9 (02) :748-769
[9]   SUPERRADIANT EMISSION AND OPTICAL DEPHASING IN J-AGGREGATES [J].
FIDDER, H ;
KNOESTER, J ;
WIERSMA, DA .
CHEMICAL PHYSICS LETTERS, 1990, 171 (5-6) :529-536
[10]   RESONANCE-LIGHT-SCATTERING STUDY AND LINE-SHAPE SIMULATION OF THE J-BAND [J].
FIDDER, H ;
WIERSMA, DA .
PHYSICAL REVIEW LETTERS, 1991, 66 (11) :1501-1504