SHORT-RANGE MAGNETIC-ORDERING IN THE HIGHLY FRUSTRATED PYROCHLORE Y2MN2O7

被引:125
作者
REIMERS, JN
GREEDAN, JE
KREMER, RK
GMELIN, E
SUBRAMANIAN, MA
机构
[1] MCMASTER UNIV,MCMASTER NUCL REACTOR,HAMILTON L8S 4M1,ONTARIO,CANADA
[2] MAX PLANCK INST FESTKORPERFORSCH,W-7000 STUTTGART 80,GERMANY
[3] DUPONT CO,EXPT STN,WILMINGTON,DE 19898
来源
PHYSICAL REVIEW B | 1991年 / 43卷 / 04期
关键词
D O I
10.1103/PhysRevB.43.3387
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The bulk magnetic susceptibility of Y2Mn2O7 is suggestive of ferromagnetic order, with THETA-C = +41(2) K, and an apparent T(c) = 20 K. However, both dc and ac susceptibility data show a broad maximum near 7 K, which is frequency and field dependent. Heat-capacity studies down to 2 K show no evidence for long-range magnetic order. Neutron-scattering data indicate the presence of both antiferromagnetic (first neighbors) and ferromagnetic (second and third neighbors) short-range correlations. These results are compared to mean-field-theory predictions for the highly frustrated 16c sites in the pyrochlore lattice. This material shows many properties in common with spin glasses in spite of the fact that there is no evidence for chemical disorder.
引用
收藏
页码:3387 / 3394
页数:8
相关论文
共 25 条
[1]   VERY LOW FIELD SUSCEPTIBILITY OF THE HIGHLY FRUSTRATED CSMNFEF6 AND CSNIFEF6 COMPOUNDS [J].
ALBA, M ;
HAMMANN, J ;
JACOBONI, C ;
PAPPA, C .
PHYSICS LETTERS A, 1982, 89 (08) :423-426
[2]   ORDERING AND ANTIFERROMAGNETISM IN FERRITES [J].
ANDERSON, PW .
PHYSICAL REVIEW, 1956, 102 (04) :1008-1013
[3]   STRUCTURE OF RBNICRF6 TYPE AND RELATION TO PYROCHLORE STRUCTURE [J].
BABEL, D .
ZEITSCHRIFT FUR ANORGANISCHE UND ALLGEMEINE CHEMIE, 1972, 387 (02) :161-&
[4]   ORDRE MAGNETIQUE A COURTE DISTANCE DANS LES SOLUTIONS SOLIDES MNXCRU-XS [J].
BERTAUT, EF ;
BURLET, P .
SOLID STATE COMMUNICATIONS, 1967, 5 (04) :279-&
[5]   FRUSTRATION EFFECTS IN THE DISORDERED SYSTEM CSMNFEF6, STUDIED BY NEUTRON-SCATTERING, AC SUSCEPTIBILITY, AND MAGNETIZATION MEASUREMENTS [J].
BEVAART, L ;
TEGELAAR, PMHL ;
VANDUYNEVELDT, AJ ;
STEINER, M .
PHYSICAL REVIEW B, 1982, 26 (11) :6150-6158
[6]   SPIN-GLASSES - EXPERIMENTAL FACTS, THEORETICAL CONCEPTS, AND OPEN QUESTIONS [J].
BINDER, K ;
YOUNG, AP .
REVIEWS OF MODERN PHYSICS, 1986, 58 (04) :801-976
[7]   PYROCHLORES .3. X-RAY NEUTRON INFRARED AND DIELECTRIC STUDIES OF A2SN2O7 STANNATES [J].
BRISSE, F ;
KNOP, O .
CANADIAN JOURNAL OF CHEMISTRY, 1968, 46 (06) :859-&
[8]  
Dai W., COMMUNICATION
[9]  
GMELIN E, 1981, CRYOGENICS, V21, P177
[10]   SPIN-GLASS-LIKE BEHAVIOR IN Y2MO2O7, A CONCENTRATED, CRYSTALLINE SYSTEM WITH NEGLIGIBLE APPARENT DISORDER [J].
GREEDAN, JE ;
SATO, M ;
XU, Y ;
RAZAVI, FS .
SOLID STATE COMMUNICATIONS, 1986, 59 (12) :895-897