THE SINGLET-TRIPLET SPLITTING OF THE PRIMARY RADICAL PAIR IN THE BACTERIAL PHOTOSYNTHETIC REACTION-CENTER

被引：24

作者：

BIXON, M ^{[1
]}

JORTNER, J ^{[1
]}

MICHELBEYERLE, ME ^{[1
]}

机构：

[1] TECH UNIV MUNICH,INST PHYS CHEM,D-85748 GARCHING,GERMANY

来源：

ZEITSCHRIFT FUR PHYSIKALISCHE CHEMIE-INTERNATIONAL JOURNAL OF RESEARCH IN PHYSICAL CHEMISTRY & CHEMICAL PHYSICS | 1993年 / 180卷

关键词：

EXCHANGE INTEGRAL; PHOTOSYNTHETIC REACTION CENTER; RADICAL PAIR; ELECTRON TRANSFER;

D O I：

10.1524/zpch.1993.180.Part_1_2.193

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

A vibronic interaction model is employed for the calculation of the dynamical properties of the primary radical pair in the bacterial photosynthetic reaction center (RC). The exchange integral and the recombination rates in the singlet and triplet channels are evaluated using the same set of parameters. This set is consistent with the sequential description of the primary charge separation.

引用

页码：193 / 208

页数：16

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