DELAY-INDUCED CHAOS IN CATALYTIC SURFACE-REACTIONS - NO REDUCTION ON PT(100)

被引:73
作者
KHRUSTOVA, N [1 ]
VESER, G [1 ]
MIKHAILOV, A [1 ]
IMBIHL, R [1 ]
机构
[1] UNIV HANNOVER,INST PHYS CHEM & ELEKTROCHEM,D-30167 HANNOVER,GERMANY
关键词
D O I
10.1103/PhysRevLett.75.3564
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Deterministic chaos has been observed in the NO + CO and NO + H-2 reactions on Pt(100). A mathematical model is proposed that explains the origin as being due to delays in the response of a population of reacting adsorbate islands globally coupled via the gas phase. The dynamical equations of this model yield a sequence of period-doubling bifurcations resulting in chaos.
引用
收藏
页码:3564 / 3567
页数:4
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