INTERPLAY OF RESONANT AND AUGER PROCESSES IN PROTON NEUTRALIZATION AFTER GRAZING SURFACE SCATTERING

被引:55
作者
ZIMNY, R
MISKOVIC, ZL
NEDELJKOVIC, NN
NEDELJKOVIC, LD
机构
[1] BORIS KIDRIC INST NUCL SCI, YU-11001 BELGRADE, YUGOSLAVIA
[2] FAC SCI & MATH, FAC PHYS, YU-11001 BELGRADE, YUGOSLAVIA
[3] INST PHYS, YU-11001 BELGRADE, YUGOSLAVIA
关键词
D O I
10.1016/0039-6028(91)90017-M
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We present model calculations for proton neutralization after grazing reflection at an aluminum surface over a wide range of projectile velocities around the Bohr or Fermi velocity. The contribution of excited hydrogen states to the neutral fraction, as well as negative-ion formation can be regarded as small in this case. Both resonant and Auger electron capture from the metallic conduction band into the 1s ground state of hydrogen as well as electron loss by resonance and Auger ionization of the ground state are taken into account on equal footing within a rate-equation approach. As a consequence, our model allows to estimate, for the first time, the effect of the particle velocity parallel to the surface plane on the relative role of resonant and Auger-type electron transfer in ion-surface neutralization. The results of our theoretical model are compared with recent experimental data for grazing scattering of protons at an Al(111) surface.
引用
收藏
页码:135 / 156
页数:22
相关论文
共 89 条
[1]   THEORY OF ION NEUTRALIZATION AT METAL-SURFACES BY SURFACE-PLASMON EXCITATION [J].
ALMULHEM, AA ;
GIRARDEAU, MD .
SURFACE SCIENCE, 1989, 210 (1-2) :138-162
[2]  
AMOS AT, 1989, ADV CHEM PHYS, V76, P335
[3]   ELECTRONIC INTERACTION OF FAST IONS WITH SURFACES [J].
ANDRA, HJ ;
ZIMNY, R ;
WINTER, H ;
HAGEDORN, H .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 1985, 9 (04) :572-585
[4]   SURFACE-PLASMON DE-EXCITATION OF MULTIPLY CHARGED IONS [J].
APELL, P .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1988, 21 (14) :2665-2673
[5]   GENERAL EXPRESSION FOR THE COULOMB INTERACTION IN THE PRESENCE OF A SURFACE [J].
APELL, SP ;
PENN, DR .
PHYSICAL REVIEW B, 1986, 34 (10) :6612-6626
[6]   CHARGE-TRANSFER INTO EXCITED-STATES OF HYDROGEN-ATOMS REFLECTED ON METAL-SURFACES [J].
BRAKO, R .
PHYSICAL REVIEW B, 1984, 30 (10) :5629-5636
[7]   THEORY OF ELECTRONIC PROCESSES IN ATOM SCATTERING FROM SURFACES [J].
BRAKO, R ;
NEWNS, DM .
REPORTS ON PROGRESS IN PHYSICS, 1989, 52 (06) :655-697
[8]   ANISOTROPIC EXCITATION OF HYDROGEN 2P AFTER GRAZING ION-SURFACE SCATTERING [J].
BRAKO, R ;
WINTER, H ;
NEWNS, DM .
EUROPHYSICS LETTERS, 1988, 7 (03) :213-218
[9]   THEORY OF CHEMISORPTION [J].
BRENIG, W ;
SCHONHAMMER, K .
ZEITSCHRIFT FUR PHYSIK, 1974, 267 (03) :201-208
[10]   MODEL FOR THE PHYSICAL ADSORPTION OF ATOMIC-HYDROGEN [J].
BRUCH, LW ;
RUIJGROK, TW .
SURFACE SCIENCE, 1979, 79 (02) :509-548