QUANTUM INTERFERENCE BETWEEN RESONANT AND NONRESONANT CONTRIBUTIONS IN NEARLY RESONANT RAMAN-SCATTERING

被引:2
作者
KINOSHITA, S [1 ]
KUSHIDA, T [1 ]
机构
[1] OSAKA UNIV, DEPT PHYS, TOYONAKA, OSAKA 560, JAPAN
来源
PHYSICAL REVIEW A | 1990年 / 42卷 / 05期
关键词
D O I
10.1103/PhysRevA.42.2751
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Time-resolved secondary-radiation spectra have been calculated for a three-level system coupled with a reservoir under pulsed-light excitation. It has been found that a dip is observed in the time profile of the secondary-radiation intensity near the resonance-excitation condition, when the spectral bandwidth of the detection system is increased. If the secondary radiation is divided into the Raman and luminescence components that are, respectively, due to the mean value and fluctuation of the photoinduced emission dipole, the dip is observed only in the former. A simple analysis reveals that this dip originates from the quantum interference between the resonant and nonresonant contributions to the Raman scattering. © 1990 The American Physical Society.
引用
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页码:2751 / 2755
页数:5
相关论文
共 15 条
[1]   TIME-RESOLVED SPECTRUM FOR RESONANT LIGHT-SCATTERING IN AN EXCITON-PHONON SYSTEM [J].
AIHARA, M ;
KOTANI, A .
SOLID STATE COMMUNICATIONS, 1983, 46 (10) :751-754
[2]   TIME AND SPECTRAL RESOLUTION IN RESONANCE SCATTERING AND RESONANCE FLUORESCENCE [J].
COURTENS, E ;
SZOKE, A .
PHYSICAL REVIEW A, 1977, 15 (04) :1588-1603
[3]   NON-MARKOVIAN EFFECT IN RESONANT LIGHT-SCATTERING - TIME-RESOLVED SPECTRUM [J].
HAMA, M ;
AIHARA, M .
PHYSICAL REVIEW A, 1987, 35 (11) :4842-4845
[4]   TRANSIENT RESONANT LIGHT-SCATTERING IN A STRONGLY COUPLED LOCALIZED-ELECTRON PHONON SYSTEM [J].
HAMA, M ;
AIHARA, M .
PHYSICAL REVIEW B, 1988, 38 (02) :1221-1227
[5]   RESONANT RAMAN-SCATTERING AND LUMINESCENCE DUE TO EXCITONIC MOLECULE [J].
HANAMURA, E ;
TAKAGAHARA, T .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 1979, 47 (02) :410-422
[6]   TIME-DEPENDENT PHENOMENA ASSOCIATED WITH RESONANT SCATTERING OF LIGHT BY PERTURBED ATOMS [J].
HUBER, DL .
PHYSICAL REVIEW B, 1970, 1 (08) :3409-&
[7]   ESTIMATION OF ULTRASHORT EXCITED-STATE LIFETIMES FROM RAMAN-TO-FLUORESCENCE INTENSITY RATIOS [J].
KINOSHITA, S ;
KUSHIDA, T .
CHEMICAL PHYSICS LETTERS, 1988, 148 (06) :502-506
[8]  
KINOSHITA S, 1988, ULTRAFAST PHENOMENA, V6, P387
[9]  
KUSHIDA T, 1989, VIBRAT SPEC, V17, P495
[10]   INTERFERENCE ANALOGY OF RAMAN-LUMINESCENCE PROBLEM AND EXPERIMENTAL DISCRIMINATION BY POLARIZATION CORRELATION [J].
KUSHIDA, T .
SOLID STATE COMMUNICATIONS, 1979, 32 (01) :33-38