EFFECT OF ADSORBED SURFACE LAYERS ON SECOND-HARMONIC LIGHT FROM SILVER

被引:51
作者
BROWN, F
MATSUOKA, M
机构
[1] Williams College, Williamstown
[2] Gordon McKay Laboratory, Harvard University, Cambridge
来源
PHYSICAL REVIEW | 1969年 / 185卷 / 03期
关键词
D O I
10.1103/PhysRev.185.985
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
It has been found that atomically clean silver surfaces generate approximately four times as much harmonic light as those subjected to adsorption. Existing theories of the nonlinear optics of metals, which are based on bulk properties, must therefore be modified to account for the surface contribution. It is hypothesized that an electric dipole contribution to the nonlinear polarization may account for the present result. © 1969 The American Physical Society.
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页码:985 / &
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