NANOSECOND REVERSE SATURABLE ABSORPTION IN CUBANELIKE TRANSITION-METAL CLUSTERS

被引:87
作者
JI, W
DU, HJ
TANG, SH
SHI, S
机构
[1] NATL UNIV SINGAPORE,DEPT CHEM ENGN,SINGAPORE 0511,SINGAPORE
[2] NATL UNIV SINGAPORE,OPT CRYSTAL LAB,SINGAPORE 0511,SINGAPORE
关键词
D O I
10.1364/JOSAB.12.000876
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We report the measurement of reverse saturable absorption in four cubanelike transition-metal clusters with nanosecond laser pulses. We also present a five-level rate-equation model in which ionization and germinate recombination are included. A comparison between the model and the measured data shows that the population of the triplet states is generated mainly through the ionization-recombination process, and triplet-triplet absorption is responsible for the measured reverse saturable absorption.
引用
收藏
页码:876 / 881
页数:6
相关论文
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