BARRIERS AND DEFORMATION IN FISSION OF CHARGED METAL-CLUSTERS

被引:26
作者
YANNOULEAS, C
LANDMAN, U
机构
[1] School of Physics, Georgia Institute of Technology, Atlanta
关键词
D O I
10.1021/j100040a002
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The influence of electronic shell effects on the barriers and channels pertaining to metal-cluster fission is studied using a shell correction method in connection with an asymmetric two-center-oscillator model potential. This approach has the advantage that the ensuing shape parametrization allows for an independent variation of the deformations of parent and daughter clusters. Results for both symmetric and asymmetric channels associated with the parent clusters Na-10(2+) and Na-18(2+) are presented. We find that barriers, which separate the parent configuration from molecular-type configurations associated with preformation of the fragments, are most important and must be considered, together with the subsequent separation process, for proper elucidation of metal-cluster fission phenomena.
引用
收藏
页码:14577 / 14581
页数:5
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