DECAY DYNAMICS OF H2O(A1B1) - EXCITATION BY 2 PHOTON-ABSORPTION AT 354.6 NM

被引:6
作者
MIKULECKY, K
GERICKE, KH
COMES, FJ
机构
来源
BERICHTE DER BUNSEN-GESELLSCHAFT-PHYSICAL CHEMISTRY CHEMICAL PHYSICS | 1991年 / 95卷 / 08期
关键词
ELEMENTARY REACTIONS; MULTIPHOTON PROCESSES; PHOTOCHEMISTRY; SPECTROSCOPY; ULTRAVIOLET;
D O I
10.1002/bbpc.19910950812
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Water was photolyzed at 177.3 nm via a two-photon excitation by a frequency-tripled Nd:YAG laser (354.6 nm). The complete product state distribution of the ejected OH product was determined by LIF. The OH is produced in the vibrational ground state exclusively. OH shows a Boltzmann-type rotational distribution with a temperature parameter of about 350 K. No preferred population of LAMBDA- or spin-orbit states was observed.
引用
收藏
页码:927 / 929
页数:3
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