Dynamics and scaling of two-dimensional polymers in a dilute solution

被引:43
作者
Falck, E [1 ]
Punkkinen, O
Vattulainen, I
Ala-Nissila, T
机构
[1] Aalto Univ, Phys Lab, POB 1100, FIN-02015 Helsinki, Finland
[2] Aalto Univ, Helsinki Univ Technol, Helsinki Inst Phys, FIN-02015 Helsinki, Finland
[3] Brown Univ, Dept Phys, Providence, RI 02912 USA
来源
PHYSICAL REVIEW E | 2003年 / 68卷 / 05期
关键词
D O I
10.1103/PhysRevE.68.050102
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
The breakdown of dynamical scaling for a dilute polymer solution in two dimensions has been suggested by Shannon and Choy [Phys. Rev. Lett. 79, 1455 (1997)]. However, we show here through extensive computer simulations that dynamical scaling holds when the relevant dynamical quantities are properly extracted from finite systems. To verify dynamical scaling, we present results based on mesoscopic simulations in two dimensions for a polymer chain in a good solvent with full hydrodynamic interactions. We also present analytical arguments for the size dependence of the diffusion coefficient and find excellent agreement with the present large-scale simulations.
引用
收藏
页码:501021 / 501024
页数:4
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