Lattice Monte Carlo simulations of the activity of supported liquid-phase catalysts Part II. Nonuniform liquid distributions

被引：5

作者：

Abramova, LA ^{[1
]}

Baranov, SP

Dulov, AA

机构：

[1] ND Zelinskii Organ Chem Inst, Moscow 117913, Russia

[2] PN Lebedev Phys Inst, Moscow 117924, Russia

来源：

APPLIED CATALYSIS A-GENERAL | 2000年 / 193卷 / 1-2期

基金：

俄罗斯基础研究基金会;

关键词：

supported liquid-phase catalysts; Monte Carlo simulations;

D O I：

10.1016/S0926-860X(99)00437-8

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We develop a lattice Monte Carlo model aimed at the analysis of the activity of supported liquid-phase catalysts. We extend the model to several cases of nonuniform liquid distributions. The predictions of the model are compared with experimental results and they demonstrate a good agreement with the latter. (C) 2000 Elsevier Science B.V. All rights reserved.

引用

页码：251 / 256

页数：6

共 8 条

[1]

Abramova LA, 2000, APPL CATAL A-GEN, V193, P243, DOI 10.1016/S0926-860X(99)00436-6

[2] SUPPORTED LIQUID-PHASE CATALYSIS .3. EXPERIMENTAL EVALUATION OF THE DIFFUSION-REACTION MODEL [J].

DATTA, R ;

RYDANT, J ;

RINKER, RG .

JOURNAL OF CATALYSIS, 1985, 95 (01) :202-208

[3] SUPPORTED LIQUID-PHASE CATALYSIS .1. A THEORETICAL-MODEL FOR TRANSPORT AND REACTION [J].

DATTA, R ;

RINKER, RG .

JOURNAL OF CATALYSIS, 1985, 95 (01) :181-192

[4]

DEBELOQUI MSR, 1989, THESIS U HANNOVER

[5] SULFUR-DIOXIDE OXIDATION ON SUPPORTED MOLTEN V2O5-K2S2O7 CATALYST - INFLUENCE OF LIQUID DIFFUSION RESISTANCE [J].

LIVBJERG, H ;

JENSEN, KF ;

VILLADSEN, J .

JOURNAL OF CATALYSIS, 1976, 45 (02) :216-230

[6] THEORETICAL FOUNDATION OF CLUSTER FORMATION IN SUPPORTED LIQUID-PHASE CATALYSTS [J].

LIVBJERG, H ;

CHRISTENSEN, TS ;

HANSEN, TT ;

VILLADSEN, J .

SADHANA-ACADEMY PROCEEDINGS IN ENGINEERING SCIENCES, 1987, 10 :185-216

[7]

POLYAKOVA GM, 1971, KINET KATAL, V12, P666

[8] SUPPORTED LIQUID-PHASE CATALYSTS [J].

VILLADSEN, J ;

LIVBJERG, H .

CATALYSIS REVIEWS-SCIENCE AND ENGINEERING, 1978, 17 (02) :203-272

← 1 →