Exciton spin relaxation in quasiresonantly excited CdTe/ZnTe self-assembled quantum dots

We study exciton spin-relaxation in CdTe self-assembled quantum dots (QDs) by using polarized photoluminescence (PL) spectroscopy in magnetic field. Experiments on single CdTe QDs and on large QD ensembles show that by combining LO phonon-assisted absorption with circularly polarized excitation, spin-polarized excitons are photoexcited directly into the ground states of QDs. We find that for single symmetric QDs at B=0 T, where the exciton levels are degenerate, the spins randomize very rapidly, so that no net spin polarization is observed. In contrast, when this degeneracy is lifted by only a fraction of a Kelvin through the application of small magnetic fields, optically created spin-polarized excitons maintain their polarization on a time scale much longer than the exciton recombination time. Similar behaviors are found in a large ensemble of CdTe QDs. Finally, due to strong electronic confinement in CdTe QDs, the large spin polarization of excitons shows no dependence on the number of LO phonons emitted between the virtual state and the ground state of the exciton.