Mobility, turnover and storage of pollutants in soils, sediments and waters: achievements and results of the EU project AquaTerra. A review

被引:35
作者
Barth, J. A. C. [1 ]
Grathwohl, P. [1 ]
Fowler, H. J. [2 ]
Bellin, A. [3 ]
Gerzabek, M. H. [4 ]
Lair, G. J. [4 ]
Barcelo, D. [5 ]
Petrovic, M. [5 ]
Navarro, A. [5 ]
Negrel, Ph. [6 ]
Petelet-Giraud, E. [6 ]
Darmendrail, D. [6 ]
Rijnaarts, H. [7 ]
Langenhoff, A. [7 ]
de Weert, J. [7 ]
Slob, A. [7 ]
van der Zaan, B. M. [7 ]
Gerritse, J. [7 ]
Frank, E. [8 ]
Gutierrez, A. [6 ]
Kretzschmar, R. [9 ]
Gocht, T. [1 ]
Steidle, D. [1 ]
Garrido, F. [6 ]
Jones, K. C. [10 ]
Meijer, S. [10 ]
Moeckel, C. [10 ]
Marsman, A. [7 ]
Klaver, G.
Vogel, T. [11 ]
Buerger, C. [1 ]
Kolditz, O. [12 ]
Broers, H. P. [7 ]
Baran, N. [6 ]
Joziasse, J. [7 ]
von Tuempling, W. [12 ]
Van Gaans, P. [7 ]
Merly, C. [6 ]
Chapman, A. [13 ]
Brouyere, S. [14 ]
Aguilar, J. Batlle [14 ]
Orban, Ph. [14 ]
Tas, N. [15 ]
Smidt, H. [15 ]
机构
[1] Univ Tubingen, Ctr Appl Geosci, D-72076 Tubingen, Germany
[2] Univ Newcastle, Sch Civil Engn & Geosci, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England
[3] Univ Trent, Dept Civil & Environm Engn, I-38050 Trento, Italy
[4] Univ Bodenkultur Wien, A-1190 Vienna, Austria
[5] CSIC, Inst Invest Quim & Ambientales Barcelona, Barcelona 8034, Spain
[6] Bur Rech Geol & Minieres, F-45060 Orleans, France
[7] Netherlands Org Appl Sci Res, NL-3508 TA Utrecht, Netherlands
[8] Attempto Serv GmbH, D-72072 Tubingen, Germany
[9] ETH, Dept Environm Sci, Inst Biogeochem & Pollutant Dynam, CHN, CH-8092 Zurich, Switzerland
[10] Univ Lancaster, Dept Environm Sci, Inst Environm & Nat Sci, Lancaster LA1 4YQ, England
[11] Czech Tech Univ, Dept Hydraul & Hydrol, Fac Civil Engn, Prague 16629, Czech Republic
[12] Umweltforschungszentrum Leipzig, Dept Inland Water Res, Dept Aquat Chem & Chemometr, D-39114 Magdeburg, Germany
[13] r3 Environm Technol Ltd, Reading RG4 8NN, Berks, England
[14] Univ Liege, GEOMAC Dept, B-4000 Liege, Belgium
[15] Wageningen Univ, Microbiol Lab, NL-6703 HB Wageningen, Netherlands
基金
英国工程与自然科学研究理事会;
关键词
contaminants; organic; inorganic; European river basins; climate change; sorption; biodegradation; soil; sediment; ground- and surface water; heavy metals; review; pesticides; atrazine; isoproturon; alkyphenol; acetochlor; chlortoluron; organochlorine; Br diphenyl ethers; drugs; TOF mass spectrometry; 87Sr; EBRO RIVER-BASIN; POLYCYCLIC AROMATIC-HYDROCARBONS; POLYBROMINATED DIPHENYL ETHERS; BROMINATED FLAME RETARDANTS; QUANTITATIVE-ANALYSIS; TEMPORAL VARIABILITY; GROUNDWATER QUALITY; ORGANIC POLLUTANTS; METAL AVAILABILITY; HEAVY-METALS;
D O I
10.1051/agro:2007060
中图分类号
S3 [农学(农艺学)];
学科分类号
0901 ;
摘要
AquaTerra is one of the first environmental projects within the 6th Framework program by the European Commission. It began in June 2004 with a multidisciplinary team of 45 partner organizations from 13 EU countries, Switzerland, Serbia, Romania and Montenegro. Results from sampling and modeling in 4 large river basins (Ebro, Danube, Elbe and Meuse) and one catchment of the Brevilles Spring in France led to new evaluations of diffuse and hotspot input of persistent organic and metal pollutants including dynamics of pesticides and polycyclic aromatic hydrocarbons, as well as metal turnover and accumulation. While degradation of selected organic compounds could be demonstrated under controlled conditions in the laboratory, turnover of most persistent pollutants in the field seems to range from decades to centuries. First investigations of long-term cumulative and degradation effects, particularly in the context of climate change, have shown that it is also necessary to consider the predictions of more than one climate model when trying to assess future impacts. This is largely controlled by uncertainties in climate model responses. It is becoming evident, however, that changes to the climate will have important impacts on the diffusion and degradation of pollutants in space and time that are just at the start of their exploration.
引用
收藏
页码:161 / 173
页数:13
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