Direct Observation of the Proliferation of Ferroelectric Loop Domains and Vortex-Antivortex Pairs

被引:162
作者
Chae, S. C. [1 ]
Lee, N. [1 ]
Horibe, Y. [1 ]
Tanimura, M. [3 ]
Mori, S. [2 ,4 ]
Gao, B. [1 ]
Carr, S. [1 ]
Cheong, S. -W. [1 ]
机构
[1] Rutgers State Univ, Rutgers Ctr Emergent Mat, Piscataway, NJ 08854 USA
[2] Osaka Prefecture Univ, Dept Mat Sci, Sakai, Osaka 5998531, Japan
[3] NISSAN ARC Ltd, Res Dept, Yokosuka, Kanagawa 2370061, Japan
[4] CREST, JST, Sakai, Osaka 5998531, Japan
基金
美国国家科学基金会;
关键词
PHASE-TRANSITIONS; 2-DIMENSIONAL SYSTEMS; YMNO3; DENSITY; GROWTH; MODEL;
D O I
10.1103/PhysRevLett.108.167603
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We discovered stripe patterns of trimerization-ferroelectric domains in hexagonal REMnO3 (RE = Ho, ..., Lu) crystals (grown below ferroelectric transition temperatures (T-c), reaching up to 1435 degrees C), in contrast with the vortex patterns in YMnO3. These stripe patterns roughen with the appearance of numerous loop domains through thermal annealing just below T-c, but the stripe domain patterns turn to vortex-antivortex domain patterns through a freezing process when crystals cross T-c even though the phase transition appears to not be Kosterlitz-Thouless-type. The experimental systematics are compared with the results of our six-state clock model simulation and also the Kibble-Zurek mechanism for trapped topological defects.
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页数:5
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