Epitaxial stabilization of a new multiferroic hexagonal phase of TbMnO3 thin films

被引:98
作者
Lee, Jung-Hyuk
Murugavel, Pattukkannu
Ryu, Hyejin
Lee, Daesu
Jo, Ji Young
Kim, Jae Wook
Kim, Hyung Jin
Kim, Kee Hoon
Jo, Younghun
Jung, Myung-Hwa
Oh, Young Hwa
Kim, Young-Woon
Yoon, Jong-Gul
Chung, Jin-Seok
Noh, Tae Won [1 ]
机构
[1] Seoul Natl Univ, ReCOE & FPRD, Sch Phys & Astron, Seoul 151747, South Korea
[2] Seoul Natl Univ, CSCMR & FPRD, Sch Phys & Astron, Seoul 151747, South Korea
[3] Korea Basic Sci Inst, Quantum Mat Res Team, Taejon 305333, South Korea
[4] Seoul Natl Univ, Dept Mat Sci & Engn, Seoul 151747, South Korea
[5] Univ Suwon, Dept Phys, Suwon 445743, Gyunggi, South Korea
[6] Soongsil Univ, Dept Phys, Seoul 156743, South Korea
[7] Soongsil Univ, CAMDRC, Seoul 156743, South Korea
关键词
Epitaxial growth - Ferroelectricity - Interfaces (materials) - Interfacial energy - Substrates - Terbium compounds - Transmission electron microscopy;
D O I
10.1002/adma.200601621
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Multiferroic hexagonal TbMnO3 thin films have been epitaxially stabilized on substrates with hexagonal in-plane symmetry by pulsed laser deposition. The hexagonal TbMnO3 films show ferroelectricity below ca. 60 K with a remnant polarization 20 times larger compared to its orthorhombic bulk phase. In addition, these samples show an electric-field-induced antiferroelectric-to-ferroelectric phase transition.
引用
收藏
页码:3125 / +
页数:6
相关论文
共 19 条
[1]   Effect of Mn trimerization on the magnetic and dielectric properties of hexagonal YMnO3 -: art. no. 184418 [J].
Aikawa, Y ;
Katsufuji, T ;
Arima, T ;
Kato, K .
PHYSICAL REVIEW B, 2005, 71 (18)
[2]  
FEIBIG M, 2002, PHYS REV LETT, V88
[3]   Observation of coupled magnetic and electric domains [J].
Fiebig, M ;
Lottermoser, T ;
Fröhlich, D ;
Goltsev, AV ;
Pisarev, RV .
NATURE, 2002, 419 (6909) :818-820
[4]   Interaction of frustrated magnetic sublattices in ErMnO3 -: art. no. 027203 [J].
Fiebig, M ;
Degenhardt, C ;
Pisarev, RV .
PHYSICAL REVIEW LETTERS, 2002, 88 (02)
[5]  
Hill NA, 2002, J MAGN MAGN MATER, V242, P976
[6]  
Hill NA, 2000, J PHYS CHEM B, V104, P6694, DOI [10.1021/jp000114x, 10.1021/jpc00114x]
[7]   Electric polarization reversal and memory in a multiferroic material induced by magnetic fields [J].
Hur, N ;
Park, S ;
Sharma, PA ;
Ahn, JS ;
Guha, S ;
Cheong, SW .
NATURE, 2004, 429 (6990) :392-395
[8]  
IMURA T, 2005, PHYS REV B, V71
[9]   Magnetocapacitance and spin fluctuations in the geometrically frustrated magnets R2Ti2O7 (R = rare earth) -: art. no. 064422 [J].
Katsufuji, T ;
Takagi, H .
PHYSICAL REVIEW B, 2004, 69 (06)
[10]   Dielectric and magnetic anomalies and spin frustration in hexagonal RMnO3 (R = Y, Yb, and Lu) -: art. no. 104419 [J].
Katsufuji, T ;
Mori, S ;
Masaki, M ;
Moritomo, Y ;
Yamamoto, N ;
Takagi, H .
PHYSICAL REVIEW B, 2001, 64 (10)