NMR and ESCA studies of the "silica garden" Bronsted acid catalyst

被引:35
作者
Collins, C
Mann, G
Hoppe, E
Duggal, T
Barr, TL
Klinowski, J
机构
[1] Univ Cambridge, Dept Chem, Cambridge CB2 1EW, England
[2] Univ Wisconsin, Dept Mat, Surface Studies Lab, Milwaukee, WI 53201 USA
关键词
D O I
10.1039/a904058g
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The silica garden Bronsted acid catalyst is a framework aluminosilicate derived from silica by isomorphous substitution of 4-coordinate silicon by 4-coordinate aluminium. 6-coordinate aluminate cationic units and Bronsted protons balance the net charge of the polyanionic network.
引用
收藏
页码:3685 / 3687
页数:3
相关论文
共 20 条
[1]   NATURE OF THE USE OF ADVENTITIOUS CARBON AS A BINDING-ENERGY STANDARD [J].
BARR, TL ;
SEAL, S .
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A-VACUUM SURFACES AND FILMS, 1995, 13 (03) :1239-1246
[2]   ESCA STUDIES OF THE SURFACE-CHEMISTRY OF ZEOLITES [J].
BARR, TL ;
LISHKA, MA .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1986, 108 (12) :3178-3186
[3]   XPS VALENCE BAND STUDY OF ZEOLITES AND RELATED SYSTEMS .1. GENERAL-CHEMISTRY AND STRUCTURE [J].
BARR, TL ;
LI, MC ;
MOHSENIAN, M ;
LISHKA, MA .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1988, 110 (24) :7962-7975
[4]  
BARR TL, 1994, MODERN ESCA PRINCIPL, pCH8
[5]  
BARR TL, 1990, PRACTICAL SURFACE AN
[6]  
BARR TL, 1978, ACS DIV PETROL CHEM, V23, P82
[7]   ALUMINUM DISTRIBUTION AND PROPERTIES OF FAUJASITES - BASIS OF MODELS AND ZEOLITE ACIDITY [J].
BEAGLEY, B ;
DWYER, J ;
FITCH, FR ;
MANN, R ;
WALTERS, J .
JOURNAL OF PHYSICAL CHEMISTRY, 1984, 88 (09) :1744-1751
[8]   The 'silica garden': a hierarchical nanostructure [J].
Collins, C ;
Zhou, WZ ;
Mackay, AL ;
Klinowski, J .
CHEMICAL PHYSICS LETTERS, 1998, 286 (1-2) :88-92
[9]  
COLLINS C, UNPUB J PHYS CHEM
[10]   STUDY OF THE SURFACE-COMPOSITION OF ZEOLITES BY FAST ATOM BOMBARDMENT MASS-SPECTROMETRY [J].
DWYER, J ;
FITCH, FR ;
QIN, G ;
VICKERMAN, JC .
JOURNAL OF PHYSICAL CHEMISTRY, 1982, 86 (23) :4574-4578