Are vicinal metal surfaces stable?

被引:99
作者
Frenken, JWM
Stoltze, P
机构
[1] Leiden Univ, Kamerlingh Onnes Lab, NL-2300 RA Leiden, Netherlands
[2] Tech Univ Denmark, Ctr Atom Scale Mat Phys, Dept Phys, DK-2800 Lyngby, Denmark
关键词
D O I
10.1103/PhysRevLett.82.3500
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We use effective medium theory to demonstrate that the energies of many metal surfaces are lowered when these surfaces are replaced by facets with lower-index orientations. This implies that the low-temperature equilibrium shapes of many metal crystals should be heavily faceted. The predicted instability of vicinal metal surfaces is at variance with the almost generally observed stability of these surfaces. We argue that the unstable orientations undergo a defaceting transition at relatively low temperatures, driven by the high vibrational entropy of steps.
引用
收藏
页码:3500 / 3503
页数:4
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