Airborne measurements of dust layer properties, particle size distribution and mixing state of Saharan dust during SAMUM 2006

被引:149
作者
Weinzierl, Bernadett [1 ]
Petzold, Andreas [1 ]
Esselborn, Michael [1 ]
Wirth, Martin [1 ]
Rasp, Katharina [1 ]
Kandler, Konrad [2 ]
Schuetz, Lothar [3 ]
Koepke, Peter [4 ]
Fiebig, Markus [5 ]
机构
[1] Deutsch Zentrum Luft & Raumfahrt, Inst Phys Atmosphare, D-82234 Oberpfaffenhofen, Wessling, Germany
[2] Tech Univ Darmstadt, Inst Angew Geowissensch, D-64287 Darmstadt, Germany
[3] Johannes Gutenberg Univ Mainz, Inst Phys Atmosphare, D-55099 Mainz, Germany
[4] Univ Munich, Inst Meteorol, D-80333 Munich, Germany
[5] Norwegian Inst Air Res NILU, Dept Atmospher & Climate Res, N-2027 Kjeller, Norway
来源
TELLUS SERIES B-CHEMICAL AND PHYSICAL METEOROLOGY | 2009年 / 61卷 / 01期
关键词
OPTICAL-PROPERTIES; DESERT DUST; MINERAL AEROSOL; C-130; AIRCRAFT; PUERTO-RICO; SCATTERING; LIGHT; ABSORPTION; FSSP-300; NUMBER;
D O I
10.1111/j.1600-0889.2008.00392.x
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
The Saharan Mineral Dust Experiment (SAMUM) was conducted in May/June 2006 in southern Morocco. As part of SAMUM, airborne in situ measurements of the particle size distribution in the diameter range 4 nm < D-p < 100 mu m were conducted. The aerosol mixing state was determined below D-p < 2.5 mu m. Furthermore, the vertical structure of the dust layers was investigated with a nadir-looking high spectral resolution lidar (HSRL). The desert dust aerosol exhibited two size regimes of different mixing states: below 0.5 mu m, the particles had a non-volatile core and a volatile coating; larger particles above 0.5 mu m consisted of non-volatile components and contained light absorbing material. In all cases, particles larger than 10 mu m were present, and in 80% of the measurements no particles larger than 40 mu m were present. The abundance of large particles showed almost no height dependence. The effective diameter D-eff in the dust plumes investigated showed two main ranges: the first range of D-eff peaked around 5 mu m and the second range of D-eff around 8 mu m. The two ranges of D-eff suggest that it may be inadequate to use one average effective diameter or one parametrization for a typical dust size distribution.
引用
收藏
页码:96 / 117
页数:22
相关论文
共 61 条
[1]  
[Anonymous], 243 MPI MET
[2]  
ANSMANN A, 2005, J GEOPHYS RES, V110, P1
[3]   INTERPRETATION OF MEASUREMENTS MADE BY THE FORWARD SCATTERING SPECTROMETER PROBE (FSSP-300) DURING THE AIRBORNE ARCTIC STRATOSPHERIC EXPEDITION [J].
BAUMGARDNER, D ;
DYE, JE ;
GANDRUD, BW ;
KNOLLENBERG, RG .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1992, 97 (D8) :8035-8046
[4]  
Bohren C.F., 1983, Absorption and Scattering of Light by Small Particles
[5]   Application of the T-matrix method to the measurement of aspherical (ellipsoidal) particles with forward scattering optical particle counters [J].
Borrmann, S ;
Luo, BP ;
Mishchenko, M .
JOURNAL OF AEROSOL SCIENCE, 2000, 31 (07) :789-799
[6]   Size distributions and mixtures of dust and black carbon aerosol in Asian outflow: Physiochemistry and optical properties [J].
Clarke, AD ;
Shinozuka, Y ;
Kapustin, VN ;
Howell, S ;
Huebert, B ;
Doherty, S ;
Anderson, T ;
Covert, D ;
Anderson, J ;
Hua, X ;
Moore, KG ;
McNaughton, C ;
Carmichael, G ;
Weber, R .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D15) :D15S091-20
[7]   A THERMO OPTIC TECHNIQUE FOR INSITU ANALYSIS OF SIZE-RESOLVED AEROSOL PHYSICOCHEMISTRY [J].
CLARKE, AD .
ATMOSPHERIC ENVIRONMENT PART A-GENERAL TOPICS, 1991, 25 (3-4) :635-644
[8]  
DALMEIDA GA, 1983, J CLIM APPL METEOROL, V22, P233, DOI 10.1175/1520-0450(1983)022<0233:NMAVDO>2.0.CO
[9]  
2
[10]   Airborne observations of dust aerosol over the North Atlantic Ocean during ACE 2:: Indications for heterogeneous ozone destruction [J].
de Reus, M ;
Dentener, F ;
Thomas, A ;
Borrmann, S ;
Ström, J ;
Lelieveld, J .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2000, 105 (D12) :15263-15275