LiVGe2O6, an anomalous quasi-1D, S=1 system, as revealed by NMR

被引:35
作者
Gavilano, JL [1 ]
Mushkolaj, S
Ott, HR
Millet, P
Mila, F
机构
[1] ETH Honggerberg, Festkorperphys Lab, CH-8093 Zurich, Switzerland
[2] Ctr Elaborat Mat & Etud Struct, F-31055 Toulouse, France
[3] Univ Toulouse 3, Phys Quant Lab, F-31062 Toulouse, France
关键词
D O I
10.1103/PhysRevLett.85.409
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report the results of Li-7 nuclear magnetic resonance (NMR) studies of LiVGe2O6,a quasi-one-dimensional spin S = 1 model system, at low temperatures. Our data, including NMR spectra and the temperature dependence of the spin-lattice relaxation rate T-l(-1) indicate that a first-order phase transition occurs at T-c similar or equal to 23 K. The NMR response of LiVGe2O6 below T-c suggests that the ordered phase is antiferromagnetic and has unusual features. Possible reasons for this unexpected behavior are discussed.
引用
收藏
页码:409 / 412
页数:4
相关论文
共 16 条
[1]   RIGOROUS RESULTS ON VALENCE-BOND GROUND-STATES IN ANTIFERROMAGNETS [J].
AFFLECK, I ;
KENNEDY, T ;
LIEB, EH ;
TASAKI, H .
PHYSICAL REVIEW LETTERS, 1987, 59 (07) :799-802
[2]   EXPERIMENTAL-EVIDENCE FOR THE LOWEST EXCITATION MODE IN THE S = 1 HALDANE-GAP SYSTEM - HIGH-FIELD PROTON MAGNETIC-RELAXATION IN NI(C2H8N2)2NO2CLO4 [J].
FUJIWARA, N ;
GOTO, T ;
MAEGAWA, S ;
KOHMOTO, T .
PHYSICAL REVIEW B, 1992, 45 (14) :7837-7840
[4]   OBSERVATION OF THE SPIN-PEIERLS TRANSITION IN LINEAR CU2+ (SPIN-1/2) CHAINS IN AN INORGANIC COMPOUND CUGEO3 [J].
HASE, M ;
TERASAKI, I ;
UCHINOKURA, K .
PHYSICAL REVIEW LETTERS, 1993, 70 (23) :3651-3654
[5]   EXPERIMENTAL STUDIES OF ONE-DIMENSIONAL QUANTUM SPIN SYSTEMS [J].
KATSUMATA, K .
JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 1995, 140 :1595-1598
[6]   Variational and density-matrix renormalization-group studies of the frustrated antiferromagnetic Heisenberg S=1 quantum spin chain [J].
Kolezhuk, A ;
Roth, R ;
Schollwock, U .
PHYSICAL REVIEW B, 1997, 55 (14) :8928-8939
[7]   ABRUPT BUT CONTINUOUS ANTIFERROMAGNETIC TRANSITION IN NEARLY STOICHIOMETRIC LA2CUO4+DELTA [J].
MACLAUGHLIN, DE ;
VITHAYATHIL, JP ;
BROM, HB ;
DEROOY, JCJM ;
HAMMEL, PC ;
CANFIELD, PC ;
REYES, AP ;
FISK, Z ;
THOMPSON, JD ;
CHEONG, SW .
PHYSICAL REVIEW LETTERS, 1994, 72 (05) :760-763
[8]  
Mila F., UNPUB
[9]   Biquadratic interactions and spin-Peierls transition in the spin-1 chain LiVGe2O6 [J].
Millet, P ;
Mila, F ;
Zhang, FC ;
Mambrini, M ;
Van Oosten, AB ;
Pashchenko, VA ;
Sulpice, A ;
Stepanov, A .
PHYSICAL REVIEW LETTERS, 1999, 83 (20) :4176-4179
[10]   DYNAMIC STRUCTURE FACTOR [S(Q,OMEGA)] OF THE S = 1 QUASI-ONE-DIMENSIONAL HEISENBERG-ANTIFERROMAGNET - NEUTRON-SCATTERING STUDY ON AGVP2S6 [J].
MUTKA, H ;
PAYEN, C ;
MOLINIE, P ;
SOUBEYROUX, JL ;
COLOMBET, P ;
TAYLOR, AD .
PHYSICAL REVIEW LETTERS, 1991, 67 (04) :497-500