Direct transport of midlatitude stratospheric ozone into the lower troposphere and marine boundary layer of the tropical Pacific Ocean -: art. no. D23310

被引:72
作者
Cooper, OR
Stohl, A
Hübler, G
Hsie, EY
Parrish, DD
Tuck, AF
Kiladis, GN
Oltmans, SJ
Johnson, BJ
Shapiro, M
Moody, JL
Lefohn, AS
机构
[1] Univ Colorado, NOAA, Aeron Lab, Cooperat Inst Res Environm Sci, Boulder, CO 80305 USA
[2] NOAA, Climate Monitoring & Diagnost Lab, Boulder, CO 80305 USA
[3] NOAA, Univ Corp Atmospher Res, Boulder, CO 80301 USA
[4] Univ Virginia, Dept Environm Sci, Charlottesville, VA 22904 USA
[5] ASL & Associates, Helena, MT 59601 USA
关键词
D O I
10.1029/2005JD005783
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
The detailed survey of midlatitude stratospheric intrusions penetrating into the Northern Hemisphere tropics was one goal of the Pacific Sub-Tropical Jet Study 2004, conducted from Honolulu, Hawaii, during 19-29 January and 28 February to 15 March. Using the National Oceanic and Atmospheric Administration G-IV jet aircraft, instrumented with dropsondes and a 1-s resolution ozone instrument, we targeted an intrusion above Hawaii on 29 February. The data describe the strongest tropospheric ozone enhancements ever measured above Hawaii (in comparison to a 22 year ozonesonde record) and illustrate the mixing of stratospheric ozone into the midtroposphere as a result of convection triggered by the advection of relatively cold midlatitude air into the tropics. Measurements from the G-IV and Mauna Loa Observatory (3.4 km) show enhanced ozone in the lower troposphere, indicating that the remnants of the intrusion reached these levels. This conclusion is supported by a study using a stratospheric ozone tracer generated by the FLEXPART Lagrangian particle dispersion model. This paper also describes a similar intrusion that enhanced ozone at Mauna Loa on 10 March, as well as Honolulu, which is located in the marine boundary layer. G-IV flights in and out of Honolulu measured enhanced ozone associated with this event on several occasions. The 10 March event transported an estimated 1.75 Tg of ozone into the tropical troposphere, and we suggest that stratospheric intrusions that break away from the polar jet stream as they advect into the tropics are more effective at transporting ozone into the troposphere than intrusions that remain close to the polar jet stream in midlatitudes. Analysis of the dynamic conditions indicates that the frequency of stratospheric intrusions was not anomalous during January-March 2004. While the 10 March event was by itself an extreme event, strong stratospheric intrusions can be expected to influence the tropical lower troposphere in any year.
引用
收藏
页码:1 / 15
页数:15
相关论文
共 63 条
[1]   VERTICAL PROFILES OF TROPOSPHERIC GASES - CHEMICAL CONSEQUENCES OF STRATOSPHERIC INTRUSIONS [J].
BAMBER, DJ ;
HEALEY, PGW ;
JONES, BMR ;
PENKETT, SA ;
TUCK, AF ;
VAUGHAN, G .
ATMOSPHERIC ENVIRONMENT, 1984, 18 (09) :1759-1766
[2]   Planetary-scale tropopause folds in the southern subtropics [J].
Baray, JL ;
Daniel, V ;
Ancellet, G ;
Legras, B .
GEOPHYSICAL RESEARCH LETTERS, 2000, 27 (03) :353-356
[3]   Dynamical study of a tropical cut-off low over South Africa, and its impact on tropospheric ozone [J].
Baray, JL ;
Baldy, S ;
Diab, RD ;
Cammas, JP .
ATMOSPHERIC ENVIRONMENT, 2003, 37 (11) :1475-1488
[4]   Transport of ozone to the surface by convective downdrafts at night [J].
Betts, AK ;
Gatti, LV ;
Cordova, AM ;
Dias, MAFS ;
Fuentes, JD .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2002, 107 (D20) :LBA13-1
[5]   Large-scale air mass characteristics observed over western Pacific during summertime [J].
Browell, EV ;
Fenn, MA ;
Butler, CF ;
Grant, WB ;
Merrill, JT ;
Newell, RE ;
Bradshaw, JD ;
Sandholm, ST ;
Anderson, BE ;
Bandy, AR ;
Bachmeier, AS ;
Blake, DR ;
Davis, DD ;
Gregory, GL ;
Heikes, BG ;
Kondo, Y ;
Liu, SC ;
Rowland, FS ;
Sachse, GW ;
Singh, HB ;
Talbot, RW ;
Thornton, DC .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1996, 101 (D1) :1691-1712
[6]   Large-scale air mass characteristics observed over the remote tropical Pacific Ocean during March-April 1999: Results from PEM-Tropics B field experiment [J].
Browell, EV ;
Fenn, MA ;
Butler, CF ;
Grant, WB ;
Ismail, S ;
Ferrare, RA ;
Kooi, SA ;
Brackett, VG ;
Clayton, MB ;
Avery, MA ;
Barrick, JDW ;
Fuelberg, HE ;
Maloney, JC ;
Newell, RE ;
Zhu, Y ;
Mahoney, MJ ;
Anderson, BE ;
Blake, DR ;
Brune, WH ;
Heikes, BG ;
Sachse, GW ;
Singh, HB ;
Talbot, RW .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D23) :32481-32501
[7]   On the life cycle of a stratospheric intrusion and its dispersion into polluted warm conveyor belts -: art. no. D23S09 [J].
Cooper, O ;
Forster, C ;
Parrish, D ;
Dunlea, E ;
Hübler, G ;
Fehsenfeld, F ;
Holloway, J ;
Oltmans, S ;
Johnson, B ;
Wimmers, A ;
Horowitz, L .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D23) :1-18
[8]   The North Atlantic Oscillation controls air pollution transport to the Arctic [J].
Eckhardt, S ;
Stohl, A ;
Beirle, S ;
Spichtinger, N ;
James, P ;
Forster, C ;
Junker, C ;
Wagner, T ;
Platt, U ;
Jennings, SG .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2003, 3 :1769-1778
[9]  
Emanuel K. A., 1994, Atmospheric Convection
[10]  
Emanuel KA, 1999, J ATMOS SCI, V56, P1766, DOI 10.1175/1520-0469(1999)056<1766:DAEOAC>2.0.CO