Polymer electrolyte membrane fuel cell;
Droplet behaviour;
Gas diffusion layer;
Water management;
Gas channel land area;
Hydrophobic;
Hydrophilic;
D O I:
10.1016/j.jpowsour.2008.07.031
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
We studied the interaction of a water droplet with a solid wall on a hydrophobic gas diffusion layer (GDL). Of particular interest is the stability of the droplet as a function of plate wetting properties and the potential for liquid entrapment in the GDL/land contact area. Such transport is of relevance to breakthrough dynamics and convective liquid droplet transport in polymer electrolyte membrane (PEM) fuel cell cathode gas channels. While a variety of complex coupled transport phenomena are present in the PEM fuel cell gas channel. we utilize a very simplified experimental model of the system where a droplet originally placed on a hydrophobic GDL is translated quasistatically across the GDL surface by a solid surface. Transport and entrapment are imaged using fluorescence microscopy. This work provides new insights into droplet behaviour at the GDL/land interface in a PEM fuel cell and suggests that hydrophobic land areas are preferable for mitigating the accumulation of liquid water under the land area of the gas flow channels. (C) 2008 Elsevier B.V. All rights reserved.
机构:Penn State Univ, Radiat Sci & Engn Ctr, Fuel Cell Dynam & Diagnost, University Pk, PA 16802 USA
Kowal, J. J.
;
Turhan, A.
论文数: 0引用数: 0
h-index: 0
机构:Penn State Univ, Radiat Sci & Engn Ctr, Fuel Cell Dynam & Diagnost, University Pk, PA 16802 USA
Turhan, A.
;
Heller, K.
论文数: 0引用数: 0
h-index: 0
机构:Penn State Univ, Radiat Sci & Engn Ctr, Fuel Cell Dynam & Diagnost, University Pk, PA 16802 USA
Heller, K.
;
Brenizer, J.
论文数: 0引用数: 0
h-index: 0
机构:Penn State Univ, Radiat Sci & Engn Ctr, Fuel Cell Dynam & Diagnost, University Pk, PA 16802 USA
Brenizer, J.
;
Mench, M. M.
论文数: 0引用数: 0
h-index: 0
机构:
Penn State Univ, Radiat Sci & Engn Ctr, Fuel Cell Dynam & Diagnost, University Pk, PA 16802 USAPenn State Univ, Radiat Sci & Engn Ctr, Fuel Cell Dynam & Diagnost, University Pk, PA 16802 USA
机构:
Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Kramer, D
;
Zhang, JB
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Zhang, JB
;
Shimoi, R
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Shimoi, R
;
Lehmann, E
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Lehmann, E
;
Wokaun, A
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Wokaun, A
;
Shinohara, K
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Shinohara, K
;
Scherer, GG
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
机构:
Penn State Univ, Fuel Cell Dynam & Diagnost Lab, Dept Mech & Nucl Engn, University Pk, PA 16802 USAPenn State Univ, Fuel Cell Dynam & Diagnost Lab, Dept Mech & Nucl Engn, University Pk, PA 16802 USA
Kumbur, E. C.
;
Sharp, K. V.
论文数: 0引用数: 0
h-index: 0
机构:
Penn State Univ, Fuel Cell Dynam & Diagnost Lab, Dept Mech & Nucl Engn, University Pk, PA 16802 USAPenn State Univ, Fuel Cell Dynam & Diagnost Lab, Dept Mech & Nucl Engn, University Pk, PA 16802 USA
Sharp, K. V.
;
Mench, M. M.
论文数: 0引用数: 0
h-index: 0
机构:
Penn State Univ, Fuel Cell Dynam & Diagnost Lab, Dept Mech & Nucl Engn, University Pk, PA 16802 USAPenn State Univ, Fuel Cell Dynam & Diagnost Lab, Dept Mech & Nucl Engn, University Pk, PA 16802 USA
机构:Penn State Univ, Radiat Sci & Engn Ctr, Fuel Cell Dynam & Diagnost, University Pk, PA 16802 USA
Kowal, J. J.
;
Turhan, A.
论文数: 0引用数: 0
h-index: 0
机构:Penn State Univ, Radiat Sci & Engn Ctr, Fuel Cell Dynam & Diagnost, University Pk, PA 16802 USA
Turhan, A.
;
Heller, K.
论文数: 0引用数: 0
h-index: 0
机构:Penn State Univ, Radiat Sci & Engn Ctr, Fuel Cell Dynam & Diagnost, University Pk, PA 16802 USA
Heller, K.
;
Brenizer, J.
论文数: 0引用数: 0
h-index: 0
机构:Penn State Univ, Radiat Sci & Engn Ctr, Fuel Cell Dynam & Diagnost, University Pk, PA 16802 USA
Brenizer, J.
;
Mench, M. M.
论文数: 0引用数: 0
h-index: 0
机构:
Penn State Univ, Radiat Sci & Engn Ctr, Fuel Cell Dynam & Diagnost, University Pk, PA 16802 USAPenn State Univ, Radiat Sci & Engn Ctr, Fuel Cell Dynam & Diagnost, University Pk, PA 16802 USA
机构:
Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Kramer, D
;
Zhang, JB
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Zhang, JB
;
Shimoi, R
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Shimoi, R
;
Lehmann, E
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Lehmann, E
;
Wokaun, A
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Wokaun, A
;
Shinohara, K
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Shinohara, K
;
Scherer, GG
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
机构:
Penn State Univ, Fuel Cell Dynam & Diagnost Lab, Dept Mech & Nucl Engn, University Pk, PA 16802 USAPenn State Univ, Fuel Cell Dynam & Diagnost Lab, Dept Mech & Nucl Engn, University Pk, PA 16802 USA
Kumbur, E. C.
;
Sharp, K. V.
论文数: 0引用数: 0
h-index: 0
机构:
Penn State Univ, Fuel Cell Dynam & Diagnost Lab, Dept Mech & Nucl Engn, University Pk, PA 16802 USAPenn State Univ, Fuel Cell Dynam & Diagnost Lab, Dept Mech & Nucl Engn, University Pk, PA 16802 USA
Sharp, K. V.
;
Mench, M. M.
论文数: 0引用数: 0
h-index: 0
机构:
Penn State Univ, Fuel Cell Dynam & Diagnost Lab, Dept Mech & Nucl Engn, University Pk, PA 16802 USAPenn State Univ, Fuel Cell Dynam & Diagnost Lab, Dept Mech & Nucl Engn, University Pk, PA 16802 USA