Re-construction and updating our understanding on the global weapons tests 137Cs fallout

被引:156
作者
Aoyama, M
Hirose, K
Igarashi, Y
机构
[1] Geochemical Research Department, Meteorological Research Institute
来源
JOURNAL OF ENVIRONMENTAL MONITORING | 2006年 / 8卷 / 04期
基金
新加坡国家研究基金会;
关键词
D O I
10.1039/b512601k
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
Global nuclear weapons tests fallout of Cs-137 in the northern hemisphere has been documented in the UNSCEAR ( United Nations Scientific Committee on the Effect of Atomic Radiation) reports. However, many questions have arisen during the past three to four decades; e. g. the water column inventory of Cs-137 in the North Pacific Ocean was two to three time higher than the cumulative decay corrected fallout at the same latitude as stated in the UNSCEAR reports. Here we show more precise spatial distribution of global Cs-137 fallout primarily on the basis of global measurements in rain, seawater and soil, as data from 101 x 101 grids. A typical feature of geographical distribution is that two high global Cs-137 fallout areas exist in the northern hemisphere, where the highest Cs-137 fallout was observed in the globe. These areas correspond to crossovers of areas where larger precipitation amounts were expected and where higher stratosphere - troposphere exchange was expected. Our new estimate of 765 +/- 79 PBq as global Cs-137 fallout for the northern hemisphere is 1.4 times higher than that of 545 PBq in the UNSCEAR reports.
引用
收藏
页码:431 / 438
页数:8
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