Photoinduced transient stark spectroscopy in organic semiconductors: A method for charge mobility determination in the picosecond regime

被引：70

作者：

Cabanillas-Gonzalez, J ^{[1
]}

Virgili, T

Gambetta, A

Lanzani, G

Anthopoulos, TD

de Leeuw, DM

机构：

[1] Politecn Milan, IFN, CNR, Dipartimento Fis,ULTRAS,INFM, I-20133 Milan, Italy

[2] Univ London Imperial Coll Sci & Technol, Dept Phys, Blackett Lab, London SW7 2BW, England

[3] Philips Res Labs, NL-5656 AA Eindhoven, Netherlands

来源：

PHYSICAL REVIEW LETTERS | 2006年 / 96卷 / 10期

关键词：

D O I：

10.1103/PhysRevLett.96.106601

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

Subpicosecond photoinduced Stark spectroscopy experiments are carried out for measuring charge carrier mobility in organic semiconductors. The technique is demonstrated in state-of-art devices based on methanofullerene. The transient mobility of photogenerated charge carriers is measured in the picosecond time domain. Electric field dependent mobility is observed from the earliest time scales. In addition, two distinct transport regimes are revealed: a short-lived state, approximately 10 ps, of high mobility and a transient towards the trap limited transport, associated with the mesoscopic structure of the medium.

引用

页码：1 / 4

页数：4

共 30 条

[1] Organic complementary-like inverters employing methanofullerene-based ambipolar field-effect transistors
Anthopoulos, TD
de Leeuw, DM
Cantatore, E
Setayesh, S
Meijer, EJ
Tanase, C
Hummelen, JC
Blom, PWM
[J]. APPLIED PHYSICS LETTERS, 2004, 85 (18) : 4205 - 4207
[2] Ambipolar organic field-effect transistors based on a solution-processed methanofullerene
Anthopoulos, TD
Tanase, C
Setayesh, S
Meijer, EJ
Hummelen, JC
Blom, PWM
de Leeuw, DM
[J]. ADVANCED MATERIALS, 2004, 16 (23-24) : 2174 - +
[3] CHARGE TRANSPORT IN DISORDERED ORGANIC PHOTOCONDUCTORS - A MONTE-CARLO SIMULATION STUDY
BASSLER, H
[J]. PHYSICA STATUS SOLIDI B-BASIC RESEARCH, 1993, 175 (01): : 15 - 56
[4] Two-step field-induced singlet dissociation in a fluorene trimer
Cabanillas-Gonzalez, J
Antognazza, MR
Virgili, T
Lanzani, G
Gadermaier, C
Sonntag, M
Strohriegl, P
[J]. PHYSICAL REVIEW B, 2005, 71 (15)
[5] TRANSIENT SPECTROSCOPY OF EXCITONS AND POLARONS IN C-60 FILMS FROM FEMTOSECONDS TO MILLISECONDS
DICK, D
WEI, X
JEGLINSKI, S
BENNER, RE
VARDENY, ZV
MOSES, D
SRDANOV, VI
WUDL, F
[J]. PHYSICAL REVIEW LETTERS, 1994, 73 (20) : 2760 - 2763
[6] Dimitrakopoulos CD, 2002, ADV MATER, V14, P99, DOI 10.1002/1521-4095(20020116)14:2<99::AID-ADMA99>3.0.CO
[7] 2-9
[8] MOBILITY OF CHARGE-CARRIERS IN VAPOR-PHASE GROWN C-60 SINGLE-CRYSTAL
FRANKEVICH, E
MARUYAMA, Y
OGATA, H
[J]. CHEMICAL PHYSICS LETTERS, 1993, 214 (01) : 39 - 44
[9] Electroluminescence in conjugated polymers
Friend, RH
Gymer, RW
Holmes, AB
Burroughes, JH
Marks, RN
Taliani, C
Bradley, DDC
Dos Santos, DA
Brédas, JL
Lögdlund, M
Salaneck, WR
[J]. NATURE, 1999, 397 (6715) : 121 - 128
[10] Direct observation of ultrafast field-induced charge generation in ladder-type poly(para-phenylene)
Graupner, W
Cerullo, G
Lanzani, G
Nisoli, M
List, EJW
Leising, G
De Silvestri, S
[J]. PHYSICAL REVIEW LETTERS, 1998, 81 (15) : 3259 - 3262

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