Polarizable particle aggregation under rotating magnetic fields using scattering dichroism

被引:73
作者
Melle, S
Calderón, OG
Fuller, GG [1 ]
Rubio, MA
机构
[1] Stanford Univ, Dept Chem Engn, Stanford, CA 94305 USA
[2] Univ Nacl Educ Distancia, Dept Fis Fundamental, Madrid 28040, Spain
[3] Univ Complutense Madrid, Dept Opt, Madrid 28040, Spain
关键词
magnetorheological suspensions; rotating fields; scattering dichroism;
D O I
10.1006/jcis.2001.8087
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We used scattering dichroism to study the dynamics of Bipolar chains induced in magnetorheological suspensions under rotating magnetic fields. Both the dichroism (proportional to the total number of aggregated particles) and the phase lag show different behavior below and above a cross-over frequency. The cross-over frequency depends linearly on both the square of the magnetization and the inverse of the viscosity. The Mason number (ratio of viscous to magnetic forces) governs the dynamics. Therefore, there is a cross-over Mason number below which the dichroism remains almost constant and above which the rotation of the field prevents the particle aggregation process from taking place. Our experimental results have been compared with particle dynamics simulations showing good agreement. (C) 2002 Elsevier Science (USA).
引用
收藏
页码:200 / 209
页数:10
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