Coincidence imaging of Coulomb explosion of CS2 in intense laser fields

被引：114

作者：

Hasegawa, H ^{[1
]}

Hishikawa, A ^{[1
]}

Yamanouchi, K ^{[1
]}

机构：

[1] Univ Tokyo, Sch Sci, Dept Chem, Bunkyo Ku, Tokyo 1130033, Japan

来源：

CHEMICAL PHYSICS LETTERS | 2001年 / 349卷 / 1-2期

关键词：

D O I：

10.1016/S0009-2614(01)01087-9

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The coincidence imaging technique is applied to direct determination of the momentum vectors of all the fragment ions produced through every event of the Coulomb explosion of a single molecular ion, CS22+ (z = 2-4) formed in intense laser of CS23+ just fields (similar to 60 fs, 0.36 x 10(15) W/cm(2)). The molecular structure I before the Coulomb explosion, CS23+ --> S+ + C+ + S+, is reconstructed from the measured momentum vectors of the fragment ions. The mean C-S bond length of <r > = 2.5 Angstrom and the azimuthally averaged S-C-S bond angle, < gamma > = 145 degrees, thus determined indicate that structural deformation occurs to a large extent in the intense laser fields. (C) 2001 Elsevier Science B.V. All rights reserved.

引用

页码：57 / 63

页数：7

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