Formation of nanoporous platinum by selective anodic dissolution of PtZn surface alloy in a Lewis acidic zinc chloride-1-ethyl-3-methylimidazolium chloride ionic liquid

被引:93
作者
Huang, JF [1 ]
Sun, IW [1 ]
机构
[1] Natl Cheng Kung Univ, Dept Chem, Tainan 70101, Taiwan
关键词
D O I
10.1021/cm030462m
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A simple electrochemical strategy is described to prepare high surface area nanostructured platinum electrode by alloying and de-alloying of PtZn in a Lewis acidic ZnCl2-1-ethyl-3-methylimidazolium chloride ionic liquid. The resulting Pt electrode showed significantly enhanced current for hydrogen and methanol redox reactions, due to the increased surface area.
引用
收藏
页码:1829 / 1831
页数:3
相关论文
共 19 条
[1]   Mesoporous platinum films from lyotropic liquid crystalline phases [J].
Attard, GS ;
Bartlett, PN ;
Coleman, NRB ;
Elliott, JM ;
Owen, JR ;
Wang, JH .
SCIENCE, 1997, 278 (5339) :838-840
[2]   Catalysis by gold [J].
Bond, GC ;
Thompson, DT .
CATALYSIS REVIEWS-SCIENCE AND ENGINEERING, 1999, 41 (3-4) :319-388
[3]   Electrodeposition of cobalt and zinc-cobalt alloys from a lewis acidic zinc chloride-1-ethyl-3 methylimidazolium chloride molten salt [J].
Chen, PY ;
Sun, IW .
ELECTROCHIMICA ACTA, 2001, 46 (08) :1169-1177
[4]   On-line characterization of platinum/graphite catalysts during liquid phase oxidations using cyclic voltammetry [J].
deBruijn, FA ;
Kuster, BFM ;
Marin, GB .
APPLIED CATALYSIS A-GENERAL, 1996, 145 (1-2) :351-374
[5]   Ionic liquids. Green solvents for the future [J].
Earle, MJ ;
Seddon, KR .
PURE AND APPLIED CHEMISTRY, 2000, 72 (07) :1391-1398
[6]   ELECTROCHEMISTRY OF METHANOL AT LOW-INDEX CRYSTAL PLANES OF PLATINUM - AN INTEGRATED VOLTAMMETRIC AND CHRONOAMPEROMETRIC STUDY [J].
HERRERO, E ;
FRANASZCZUK, K ;
WIECKOWSKI, A .
JOURNAL OF PHYSICAL CHEMISTRY, 1994, 98 (19) :5074-5083
[7]   Lewis acidity dependency of the electrochemical window of zinc chloride-1-ethyl-3-methylimidazolium chloride ionic liquids [J].
Hsiu, SI ;
Huang, JF ;
Sun, IW ;
Yuan, CH ;
Shiea, J .
ELECTROCHIMICA ACTA, 2002, 47 (27) :4367-4372
[8]   Electrochemical studies of tin in zinc chloride-1-ethyl-3-methylimidazolium chloride ionic liquids [J].
Huang, JF ;
Sun, IW .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2003, 150 (06) :E299-E306
[9]   Electrochemical study of cadmium in acidic zinc chloride-1-ethyl-3-methylimidazolium chloride ionic liquids [J].
Huang, JF ;
Sun, IW .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2002, 149 (09) :E348-E355
[10]   A lost-wax approach to monodisperse colloids and their crystals [J].
Jiang, P ;
Bertone, JF ;
Colvin, VL .
SCIENCE, 2001, 291 (5503) :453-457