Visualization and quantification of cathode channel flooding in PEM fuel cells

被引:261
作者
Hussaini, Irfan S. [1 ,2 ]
Wang, Chao-Yang [1 ,2 ]
机构
[1] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA
[2] Penn State Univ, ECEC, University Pk, PA 16802 USA
关键词
Polymer electrolyte fuel cell; Visualization; Two-phase flow; Channel flooding; Water management; Flow map; LIQUID-WATER; 2-PHASE FLOW; TRANSPORT;
D O I
10.1016/j.jpowsour.2008.11.030
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
An understanding of two-phase flow mechanisms in micro-channels is critical to water management in fuel cell applications. In this work,an in situ visualization study of cathode flooding in an operating fuel cell is presented. Gas relative humidities of 26%, 42% and 66%, current densities of 0.2. 0.5 and 0.8 A cm(-2) and flow stoichiometries ranging from 2 to 4 are used in this study which represent typical operating conditions for automotive applications. Results are presented in the form of a flow map depicting various two-phase flow patterns. The impact of flooding is also presented in terms of measurable parameters like two-phase pressure drop coefficient and voltage loss. A new parameter called wetted area ratio is introduced to characterize channel flooding and liquid water coverage on a gas diffusion layer, and its repeatability with multiple tests is demonstrated. (C) 2008 Elsevier B.V. All rights reserved.
引用
收藏
页码:444 / 451
页数:8
相关论文
共 24 条
[1]   FLOW PATTERN CHARACTERIZATION IN 2-PHASE FLOW BY ELECTRICAL CONDUCTANCE PROBE [J].
BARNEA, D ;
SHOHAM, O ;
TAITEL, Y .
INTERNATIONAL JOURNAL OF MULTIPHASE FLOW, 1980, 6 (05) :387-397
[2]   Neutron imaging technique for in situ measurement of water transport gradients within Nafion in polymer electrolyte fuel cells [J].
Bellows, RJ ;
Lin, MY ;
Arif, M ;
Thompson, AK ;
Jacobson, D .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1999, 146 (03) :1099-1103
[3]   IN-SITU MEMBRANE RESISTANCE MEASUREMENTS IN POLYMER ELECTROLYTE FUEL-CELLS BY FAST AUXILIARY CURRENT PULSES [J].
BUCHI, FN ;
MAREK, A ;
SCHERER, GG .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1995, 142 (06) :1895-1901
[4]  
Carey VP., 2020, LIQUID VAPOR PHASE C
[5]  
Carrette L, 2001, FUEL CELLS, V1, P5, DOI 10.1002/1615-6854(200105)1:1<5::AID-FUCE5>3.0.CO
[6]  
2-G
[7]   Electrical test methods for on-line fuel cell ohmic resistance measurement [J].
Cooper, K. R. ;
Smith, M. .
JOURNAL OF POWER SOURCES, 2006, 160 (02) :1088-1095
[8]   Development of a residence time distribution method for proton exchange membrane fuel cell evaluation [J].
Diep, J. ;
Kiel, D. ;
St-Pierre, J. ;
Wong, A. .
CHEMICAL ENGINEERING SCIENCE, 2007, 62 (03) :846-857
[9]  
Faghri A., 2006, Transport Phenomena in Multiphase Systems with Phase Change
[10]   WATER AND THERMAL MANAGEMENT IN SOLID-POLYMER-ELECTROLYTE FUEL-CELLS [J].
FULLER, TF ;
NEWMAN, J .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1993, 140 (05) :1218-1225