Theoretical comparison between field emission from single-wall and multi-wall carbon nanotubes

被引:45
作者
Mayer, A
Miskovsky, NM
Cutler, PH
机构
[1] Fac Univ Notre Dame Paix, Lab Phys Solide, B-5000 Namur, Belgium
[2] Penn State Univ, Dept Phys, Davey Lab 104, University Pk, PA 16802 USA
关键词
D O I
10.1103/PhysRevB.65.155420
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We present three-dimensional simulations of field emission from single-wall and multi-wall carbon nanotubes. The structures considered are the metallic ideally open (5,5), (10,10), (15,15) and (5,5)@(10,10)@(15,15) nanotubes. For the multi-wall structure, flat and convex terminations are considered. The scattering calculations are achieved using a transfer-matrix methodology and band-structure effects result from using pseudopotentials and repeating periodically a basic unit of the nanotubes. The electronic emission from the single-wall nanotubes considered is found to decrease linearly with the radius of the tube. Multi-wall nanotubes are better emitters than single walls, the current extracted from multi-wall structures being higher than the total current obtained by considering their single-wall layers separately. The current emitted from a multi-wall structure is still increased when the termination is convex (instead of flat). The reduced polarizability of multi-wall nanotubes (compared to single-wall structures) is an important aspect for explaining their field-emission properties.
引用
收藏
页码:1554201 / 1554206
页数:6
相关论文
共 28 条
[1]   Theoretical study of field emission by single-wall carbon nanotubes [J].
Adessi, C ;
Devel, M .
PHYSICAL REVIEW B, 2000, 62 (20) :13314-13317
[2]  
ADESSI C, IN PRESS J VAC SCI B
[3]   STRUCTURAL-ENERGY CALCULATIONS BASED ON NORM-CONSERVING PSEUDOPOTENTIALS AND LOCALIZED GAUSSIAN-ORBITALS [J].
BACHELET, GB ;
GREENSIDE, HS ;
BARAFF, GA ;
SCHLUTER, M .
PHYSICAL REVIEW B, 1981, 24 (08) :4745-4752
[4]   Field emission from carbon nanotubes:: perspectives for applications and clues to the emission mechanism [J].
Bonard, JM ;
Salvetat, JP ;
Stöckli, T ;
Forró, L ;
Châtelain, A .
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 1999, 69 (03) :245-254
[5]   Electronic structure and localized states at carbon nanotube tips [J].
Carroll, DL ;
Redlich, P ;
Ajayan, PM ;
Charlier, JC ;
Blase, X ;
DeVita, A ;
Car, R .
PHYSICAL REVIEW LETTERS, 1997, 78 (14) :2811-2814
[6]   Unique characteristics of cold cathode carbon-nanotube-matrix field emitters [J].
Collins, PG ;
Zettl, A .
PHYSICAL REVIEW B, 1997, 55 (15) :9391-9399
[7]   Electronic structure at carbon nanotube tips [J].
De Vita, A ;
Charlier, JC ;
Blase, X ;
Car, R .
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 1999, 68 (03) :283-286
[8]   Nanotube electronic states observed with thermal field emission electron spectroscopy [J].
Dean, KA ;
Groening, O ;
Küttel, OM ;
Schlapbach, L .
APPLIED PHYSICS LETTERS, 1999, 75 (18) :2773-2775
[9]   A CARBON NANOTUBE FIELD-EMISSION ELECTRON SOURCE [J].
DEHEER, WA ;
CHATELAIN, A ;
UGARTE, D .
SCIENCE, 1995, 270 (5239) :1179-1180
[10]  
DRESSELHAUS MS, 2000, OPTICAL ELECT PROPER, P236